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Articles 1951 - 1980 of 8897

Full-Text Articles in Physical Sciences and Mathematics

Progress In Solar Photocatalytic Hydrogen Production, Zhi Wu, Lan Sun, Chang-Jian Lin Oct 2019

Progress In Solar Photocatalytic Hydrogen Production, Zhi Wu, Lan Sun, Chang-Jian Lin

Journal of Electrochemistry

With the rapid development of human society and dramatically consumption of traditional energy, energy shortage and environmental pollution have become an important factor restricting the sustainable development of human society. At present, the development of clean and environmentally friendly renewable energy system has drawn much attention and becomes an important priority stratagem in the world. In many green and sustainable new energy projects, semiconductor-based photocatalytic hydrogen production technology which utilizes the available clean and renewable solar energy to prepare clean hydrogen energy is excepted to solve the crisis of energy shortage and environmental pollution, has become one of the most …


Pd Nanoparticles Supported On The Etched Ni Foams As High-Performance Electrocatalysts For Direct Ethanol Fuel Cells, Chi Zhang, Cheng-Fei Li, Gao-Ren Li Oct 2019

Pd Nanoparticles Supported On The Etched Ni Foams As High-Performance Electrocatalysts For Direct Ethanol Fuel Cells, Chi Zhang, Cheng-Fei Li, Gao-Ren Li

Journal of Electrochemistry

The development of non-Pt anode electrocatalysts with high activity and long-term durability at low cost for fuel cells still remains enormous challenge. Here we report the Pd nanoparticles supported on Ni foams etched by the mixed acids (HNO3+H2SO4+H3PO4+CH3COOH) (Pd/ME-NF) that are designed and fabricated as high-performance electrocatalysts for ethanol oxidation in alkaline media. Because of the advantages of large open space, fast electrolyte penetration/diffusion and rapid electron transfer process, the Pd/ME-NF catalysts exhibited significantly improved electrocatalytic activity and durability compared with the commercial Pd/C catalysts.


A Survey Of Distributed Data Stream Processing Frameworks, Haruna Isah, Tariq Abughofa, Sazia Mahfuz, Dharmitha Ajerla, Farhana Zulkernine, Shahzad Khan Oct 2019

A Survey Of Distributed Data Stream Processing Frameworks, Haruna Isah, Tariq Abughofa, Sazia Mahfuz, Dharmitha Ajerla, Farhana Zulkernine, Shahzad Khan

Publications and Scholarship

Big data processing systems are evolving to be more stream oriented where each data record is processed as it arrives by distributed and low-latency computational frameworks on a continuous basis. As the stream processing technology matures and more organizations invest in digital transformations, new applications of stream analytics will be identified and implemented across a wide spectrum of industries. One of the challenges in developing a streaming analytics infrastructure is the difficulty in selecting the right stream processing framework for the different use cases. With a view to addressing this issue, in this paper we present a taxonomy, a comparative …


Analog Implementation Of The Hodgkin-Huxley Model Neuron, Zachary D. Mobille, George H. Rutherford, Jordan Brandt-Trainer, Rosangela Follmann, Epaminondas Rosa Oct 2019

Analog Implementation Of The Hodgkin-Huxley Model Neuron, Zachary D. Mobille, George H. Rutherford, Jordan Brandt-Trainer, Rosangela Follmann, Epaminondas Rosa

Annual Symposium on Biomathematics and Ecology Education and Research

No abstract provided.


Effective Capacity In Wireless Networks: A Comprehensive Survey, Muhammad Amjad, Mubashir Husain Rehmani, Leila Musavian Oct 2019

Effective Capacity In Wireless Networks: A Comprehensive Survey, Muhammad Amjad, Mubashir Husain Rehmani, Leila Musavian

Publications

Low latency applications, such as multimedia communications, autonomous vehicles, and Tactile Internet are the emerging applications for next-generation wireless networks, such as 5th generation (5G) mobile networks. Existing physical layer channel models, however, do not explicitly consider quality of service (QoS) aware related parameters under specific delay constraints. To investigate the performance of low-latency applications in future networks, a new mathematical framework is needed. Effective capacity (EC), which is a link-layer channel model with QoS-awareness, can be used to investigate the performance of wireless networks under certain statistical delay constraints. In this paper, we provide a comprehensive survey on existing …


Laser-Spark Multicharged Ion Implantation System ‒ Application In Ion Implantation And Neural Deposition Of Carbon In Nickel (111), Oguzhan Balki Oct 2019

Laser-Spark Multicharged Ion Implantation System ‒ Application In Ion Implantation And Neural Deposition Of Carbon In Nickel (111), Oguzhan Balki

Electrical & Computer Engineering Theses & Dissertations

Carbon ions generated by ablation of a carbon target using an Nd:YAG laser pulse (wavelength λ = 1064 nm, pulse width τ = 7 ns, and laser fluence of 10-110 J/cm2) are characterized. Time-of-flight analyzer, a three-mesh retarding field analyzer, and an electrostatic ion energy analyzer are used to study the charge and energy of carbon ions generated by laser ablation. The dependencies of the ion signal on the laser fluence, laser focal point position relative to target surface, and the acceleration voltage are described. Up to C4+ are observed. When no acceleration voltage is applied between …


A Multicarrier Technique For Monte Carlo Simulation Of Electrothermal Transport In Nanoelectronics, Tyler J. Spence Oct 2019

A Multicarrier Technique For Monte Carlo Simulation Of Electrothermal Transport In Nanoelectronics, Tyler J. Spence

Doctoral Dissertations

The field of microelectronics plays an important role in many areas of engineering and science, being ubiquitous in aerospace, industrial manufacturing, biotechnology, and many other fields. Today, many micro- and nanoscale electronic devices are integrated into one package. e capacity to simulate new devices accurately is critical to the engineering design process, as device engineers use simulations to predict performance characteristics and identify potential issues before fabrication. A problem of particular interest is the simulation of devices which exhibit exotic behaviors due to non-equilibrium thermodynamics and thermal effects such as self-heating. Frequently, it is desirable to predict the level of …


Paper-Based Flexible Electrode Using Chemically-Modified Graphene And Functionalized Multiwalled Carbon Nanotube Composites For Electrophysiological Signal Sensing, Md Faruk Hossain, Jae Sang Heo, John Nelson, Insoo Kim Oct 2019

Paper-Based Flexible Electrode Using Chemically-Modified Graphene And Functionalized Multiwalled Carbon Nanotube Composites For Electrophysiological Signal Sensing, Md Faruk Hossain, Jae Sang Heo, John Nelson, Insoo Kim

Bioelectrics Publications

Flexible paper-based physiological sensor electrodes were developed using chemically-modified graphene (CG) and carboxylic-functionalized multiwalled carbon nanotube composites (f@MWCNTs). A solvothermal process with additional treatment was conducted to synthesize CG and f@MWCNTs to make CG-f@MWCNT composites. The composite was sonicated in an appropriate solvent to make a uniform suspension, and then it was drop cast on a nylon membrane in a vacuum filter. A number of batches (0%~35% f@MWCNTs) were prepared to investigate the performance of the physical characteristics. The 25% f@MWCNT-loaded composite showed the best adhesion on the paper substrate. The surface topography and chemical bonding of the proposed CG-f@MWCNT …


Designing An Accessible Wave Energy Conversion Device For Powering Ocean Sensors, Sophie Coppieters ‘T Wallant Oct 2019

Designing An Accessible Wave Energy Conversion Device For Powering Ocean Sensors, Sophie Coppieters ‘T Wallant

Independent Study Project (ISP) Collection

Currently, less than 5% of our oceans are comprehensively monitored and much more ocean data is needed to facilitate understanding of ocean physics, carbon cycling, and ocean ecosystems. Today, most autonomous ocean sensors are powered by primary battery, which have both limited capacity and lifetime. The goal of this research is to design a small, accessible renewable wave energy device to power autonomous free-floating ocean sensors. By designing a cheap, accessible, and simple wave energy converter, this work hopes to make ocean sensor deployment easier and cheaper for researchers, increase the lifetime of autonomous ocean sensors, and reduce the reliance …


Barriers And Opportunities To Electric Vehicle Development In Nepal, Allyson Krupa Oct 2019

Barriers And Opportunities To Electric Vehicle Development In Nepal, Allyson Krupa

Independent Study Project (ISP) Collection

As the global carbon dioxide level reaches its highest point in human history (407.4 parts per million), energy systems must transition from fossil fuel to renewable-powered sources. Since the transportation sector contributes nearly one-third of global greenhouse gas (GHG) emissions, electric mobility offers a significant opportunity to reduce GHG emissions. Globally, there has been a rise in demand for electric vehicles. In Nepal, a clean energy transition within the context of rising urbanization and air pollution is imperative for quality of life, socio-economic development, and broadly climate change mitigation/adaptation. Furthermore, Nepal’s vast hydropower potential may increase energy independence and provide …


Demonstration Of Visible And Near Infrared Raman Spectrometers And Improved Matched Filter Model For Analysis Of Combined Raman Signals, Alexander Matthew Atkinson Oct 2019

Demonstration Of Visible And Near Infrared Raman Spectrometers And Improved Matched Filter Model For Analysis Of Combined Raman Signals, Alexander Matthew Atkinson

Electrical & Computer Engineering Theses & Dissertations

Raman spectroscopy is a powerful analysis technique that has found applications in fields such as analytical chemistry, planetary sciences, and medical diagnostics. Recent studies have shown that analysis of Raman spectral profiles can be greatly assisted by use of computational models with achievements including high accuracy pure sample classification with imbalanced data sets and detection of ideal sample deviations for pharmaceutical quality control. The adoption of automated methods is a necessary step in streamlining the analysis process as Raman hardware becomes more advanced. Due to limits in the architectures of current machine learning based Raman classification models, transfer from pure …


Pulse Power Effects On Transient Plasma Ignition For Combustion, David Wayne Alderman Ii Oct 2019

Pulse Power Effects On Transient Plasma Ignition For Combustion, David Wayne Alderman Ii

Electrical & Computer Engineering Theses & Dissertations

Transient plasma ignition (TPI) uses highly non-equilibrium plasmas, driven by less than 100 nanosecond, high-voltage pulses, to initiate combustion. The effects of pulse repetition frequency (PRF) and ultrashort nanosecond rise times on TPI are investigated in this work using lean, stoichiometric, and rich air-fuel mixtures at atmospheric pressure. Experimental data show the transient plasmas driven by ultrashort rise time, high voltage pulses at high PRF’s enhance the combustion of lean or stoichiometric air-methane mixtures in a static chamber. In particular, increasing PRF enhances the combustion performance by means of reduced delay times independent of the equivalence ratio of the air-fuel …


Development Of An Autonomous Aerial Toolset For Agricultural Applications, Terrance Life Oct 2019

Development Of An Autonomous Aerial Toolset For Agricultural Applications, Terrance Life

Mahurin Honors College Capstone Experience/Thesis Projects

According to the United Nations, the world population is expected to grow from its current 7 billion to 9.7 billion by the year 2050. During this time, global food demand is also expected to increase by between 59% and 98% due to the population increase, accompanied by an increasing demand for protein due to a rising standard of living throughout developing countries. [1] Meeting this increase in required food production using present agricultural practices would necessitate a similar increase in farmland; a resource which does not exist in abundance. Therefore, in order to meet growing food demands, new methods will …


Antibacterial Properties Of Mussel-Inspired Polydopamine Coatings Prepared By A Simple Two-Step Shaking-Assisted Method, Pegah Kord Fooroshani, Elizabeth Polega, Kevin Thomson, Mohammad Saleh Akram Bhuiyan, Rattapol Pinnaratip, Mikhail Trought, Chito E. Kendrick, Yuesheng Gao, Kathryn Perrine, Lei Pan, Bruce P. Lee Sep 2019

Antibacterial Properties Of Mussel-Inspired Polydopamine Coatings Prepared By A Simple Two-Step Shaking-Assisted Method, Pegah Kord Fooroshani, Elizabeth Polega, Kevin Thomson, Mohammad Saleh Akram Bhuiyan, Rattapol Pinnaratip, Mikhail Trought, Chito E. Kendrick, Yuesheng Gao, Kathryn Perrine, Lei Pan, Bruce P. Lee

Michigan Tech Publications

A simple two-step, shaking-assisted polydopamine (PDA) coating technique was used to impart polypropylene (PP) mesh with antimicrobial properties. In this modified method, a relatively large concentration of dopamine (20 mg ml−1) was first used to create a stable PDA primer layer, while the second step utilized a significantly lower concentration of dopamine (2 mg ml−1) to promote the formation and deposition of large aggregates of PDA nanoparticles. Gentle shaking (70 rpm) was employed to increase the deposition of PDA nanoparticle aggregates and the formation of a thicker PDA coating with nano-scaled surface roughness (RMS = 110 …


Similarity-Based Chained Transfer Learning For Energy Forecasting With Big Data, Yifang Tian, Ljubisa Sehovac, Katarina Grolinger Sep 2019

Similarity-Based Chained Transfer Learning For Energy Forecasting With Big Data, Yifang Tian, Ljubisa Sehovac, Katarina Grolinger

Electrical and Computer Engineering Publications

Smart meter popularity has resulted in the ability to collect big energy data and has created opportunities for large-scale energy forecasting. Machine Learning (ML) techniques commonly used for forecasting, such as neural networks, involve computationally intensive training typically with data from a single building or a single aggregated load to predict future consumption for that same building or aggregated load. With hundreds of thousands of meters, it becomes impractical or even infeasible to individually train a model for each meter. Consequently, this paper proposes Similarity-Based Chained Transfer Learning (SBCTL), an approach for building neural network-based models for many meters by …


Academic Skill Learning And The Problem Of Complexity I: Creational Purposeful Integrated Capability At Skill (Cpics), Martin F. Gardiner Sep 2019

Academic Skill Learning And The Problem Of Complexity I: Creational Purposeful Integrated Capability At Skill (Cpics), Martin F. Gardiner

Northeast Journal of Complex Systems (NEJCS)

Physical and mental skills are intended to achieve success at acting purposefully. As capability at any skill increases, the need to adjust details of application to complexity of context and goals will increase as well. It will become more and more important to prepare mentally for what I now term Creational Purposeful Integrated Capability at Skill (CPICS). This paper develops what I mean by CPICS. Theory concerning Complex Dynamical Systems (CDS) such as the brain and other evidence points to the likelihood that the mental operations by which our brain produces any kind of skillful behavior cannot remain constant, …


A Patterning Approach To Complexity Thinking And Understanding For Students: A Case Study, Shae L. Brown Sep 2019

A Patterning Approach To Complexity Thinking And Understanding For Students: A Case Study, Shae L. Brown

Northeast Journal of Complex Systems (NEJCS)

Complexity thinking and understanding are vital skills for young people in these times of uncertainty and change. Such skills contribute to resilience and capacities for adaptivity and innovation. Within my teaching practice I have found students to be aware of complex dynamics, uncertainty and change, both in their lives and in the world. However, the current curriculum lacks language and process to conceptualise, articulate and develop complexity understanding. To address this problem, I developed and introduced a patterns-based design and process to a cohort of Australian secondary students. Comprising flowform patterning together with ecological metaphors, the design forms a conceptual …


Being In Uncertainties: An Inquiry-Based Model Leveraging Complexity In Teaching-Learning, Diane Rosen Sep 2019

Being In Uncertainties: An Inquiry-Based Model Leveraging Complexity In Teaching-Learning, Diane Rosen

Northeast Journal of Complex Systems (NEJCS)

Education is traditionally structured as a closed system, privileging result-driven methods that offer control and predictability. In recent decades this reductionist approach has been effectively challenged by interdisciplinary work in complex systems theory, revealing myriad levels of orderly disorder that make either-or, linear instruction an inadequate norm. Narrowing the broad implications of a complexity lens on education, this paper focuses on generative uncertainty in teaching-learning, a paradoxical state of epistemological and creative growth described by English poet John Keats as "the negative capability of being in uncertainties, mysteries, doubts." Opportunities to advance this potentiating capacity are especially abundant in constructivist …


Creativity As An Emergent Property Of Complex Educational System, Ceire Monahan, Mika Munakata, Ashwin Vaidya Sep 2019

Creativity As An Emergent Property Of Complex Educational System, Ceire Monahan, Mika Munakata, Ashwin Vaidya

Northeast Journal of Complex Systems (NEJCS)

The importance of creativity in education has been discussed often in the literature. While there remains no agreed-upon definition of creativity, the psychological literature points to traits of a creative person. These include the ability to think outside the box, make connections between seemingly disparate ideas, and question norms. The literature provides several examples of classroom experiments to help foster creativity in the classroom. In science and mathematics, we can start by getting students to recognize mathematics and the sciences as being creative endeavors. While these attempts are noteworthy, they are not necessarily aligned with instructional practices. In this article, …


Rethinking Educational Reforms Through A Complex Dynamical Systems Approach: Preliminary Report From An Empirical Research, Eugenia Tsiouplis, Dimitrios Stamovlasis Sep 2019

Rethinking Educational Reforms Through A Complex Dynamical Systems Approach: Preliminary Report From An Empirical Research, Eugenia Tsiouplis, Dimitrios Stamovlasis

Northeast Journal of Complex Systems (NEJCS)

Literature on educational reforms is rich of cases where changes have been attempted, without however to attain success. Likewise the Greek education system had experienced a lot of reforms, most of which have failed to make the intended changes and they attenuated shortly after their implementation or they ceased at the stage of legislative planning. On the other hand, the traditional research have failed to develop a coherent theoretical perspective and provide satisfactory interpretations of the perpetually unsuccessful reforms. This paper is part of wider project which attempts to address the above issue following the Complex Dynamical Systems (CDS) perspective, …


Editorial Introduction To The Northeast Journal Of Complex Systems (Nejcs), Hiroki Sayama, Georgi Georgiev Sep 2019

Editorial Introduction To The Northeast Journal Of Complex Systems (Nejcs), Hiroki Sayama, Georgi Georgiev

Northeast Journal of Complex Systems (NEJCS)

Editorial Introduction to the Northeast Journal of Complex Systems (NEJCS)


Fractality And Power Law Distributions: Shifting Perspectives In Educational Research, Matthijs Koopmans Sep 2019

Fractality And Power Law Distributions: Shifting Perspectives In Educational Research, Matthijs Koopmans

Northeast Journal of Complex Systems (NEJCS)

The dynamical character of education and the complexity of its constituent relationships have long been recognized, but the full appreciation of the implications of these insights for educational research is recent. Most educational research to this day tends to focus on outcomes rather than process, and rely on conventional cross-sectional designs and statistical inference methods that do not capture this complexity. This presentation focuses on two related aspects not well accommodated by conventional models, namely fractality (self-similarity, scale invariance) and power law distributions (an inverse relationship between frequency of occurrence and strength of response). Examples are presented for both phenomena …


Digital Holography Efficiency Experiments For Tactical Applications, Douglas E. Thornton Sep 2019

Digital Holography Efficiency Experiments For Tactical Applications, Douglas E. Thornton

Theses and Dissertations

Digital holography (DH) uses coherent detection and offers direct access to the complex-optical field to sense and correct image aberrations in low signal-to-noise environments, which is critical for tactical applications. The performance of DH is compared to a similar, well studied deep-turbulence wavefront sensor, the self-referencing interferometer (SRI), with known efficiency losses. Wave optics simulations with deep-turbulence conditions and noise were conducted and the results show that DH outperforms the SRI by 10's of dB due to DH's strong reference. Additionally, efficiency experiments were conducted to investigate DH system losses. The experimental results show that the mixing efficiency (37%) is …


A Harmless Wireless Quantum Alternative To Cell Phones Based On Quantum Noise, Florentin Smarandache, Robert Neil Boyd, Victor Christianto Sep 2019

A Harmless Wireless Quantum Alternative To Cell Phones Based On Quantum Noise, Florentin Smarandache, Robert Neil Boyd, Victor Christianto

Branch Mathematics and Statistics Faculty and Staff Publications

In the meantime we know that 4G and 5G technologies cause many harms to human health. Therefore, here we submit a harmless wireless quantum alternative to cell phones. It is our hope that this alternative


Targeted Germanium Ion Irradiation Of Aluminum Gallium Nitride/Gallium Nitride High Electron Mobility Transistors, Melanie E. Mace Aug 2019

Targeted Germanium Ion Irradiation Of Aluminum Gallium Nitride/Gallium Nitride High Electron Mobility Transistors, Melanie E. Mace

Theses and Dissertations

Microscale beams of germanium ions were used to target different locations of aluminum galliumnitride/gallium nitride (AlGaN/GaN) high electron mobility transistors (HEMTs) to determine location dependent radiation effects. 1.7 MeV Ge ions were targeted at the gap between the gate and the drain to observe displacement damage effects while 47 MeV Ge ions were targeted at the gate to observe ionization damage effects. Electrical data was taken pre, during, and post irradiation. To separate transient from permanent degradation, the devices were characterized after a room temperature anneal for at least 30 days. Optical images were also analyzed pre and post irradiation. …


Statuses, Challenges And Strategies In The Development Of Low-Temperature Carbon Dioxide Electroreduction Technology, Xu-Rui Zhang, Xiao-Lin Shao, Jin Yi, Yu-Yu Liu, Jiu-Jun Zhang Aug 2019

Statuses, Challenges And Strategies In The Development Of Low-Temperature Carbon Dioxide Electroreduction Technology, Xu-Rui Zhang, Xiao-Lin Shao, Jin Yi, Yu-Yu Liu, Jiu-Jun Zhang

Journal of Electrochemistry

Low-temperature carbon dioxide (CO2) electrochemical reduction technology is a hotspot for research and development in recent years as a way to reduce the negative impact of CO2 on the environment and to generate energy storage through converting electricity to low-carbon fuels. Although basic research on catalyst activity, product selectivity, and reaction mechanism has been widely reported, the design and practicality of catalytic stability and corresponding electrochemical reactor systems have not been given sufficient attention and systematic development. In this paper, two important factors affecting the development of CO2 electrochemical reduction technology in low temperature aqueous solution …


Preface To Special Issue Of Electrochemical Reduction Of Carbon Dioxide, Qing Li, Min Liu Aug 2019

Preface To Special Issue Of Electrochemical Reduction Of Carbon Dioxide, Qing Li, Min Liu

Journal of Electrochemistry

No abstract provided.


Copper-Based Compounds For Electrochemical Reduction Of Carbon Dioxide, Fan Yang, Pei-Lin Deng, You-Jia Han, Pan Jing, Bao-Yu Xia Aug 2019

Copper-Based Compounds For Electrochemical Reduction Of Carbon Dioxide, Fan Yang, Pei-Lin Deng, You-Jia Han, Pan Jing, Bao-Yu Xia

Journal of Electrochemistry

The electrochemical reduction of carbon dioxide (CO2) to useful chemicals and fuels has attracted enormous interest since the deteriorating global warming and energy shortage problems resulted from ever-increasing CO2 emission. Designing efficient catalysts is of capital significance to realize the efficient and selective conversion of CO2. Among various catalysts explored, copper-based compounds have promising potentials with acceptable efficiency for hydrocarbon production. Herein, recent advances on copper-based materials are summarized for electrochemical CO2 conversion. We intend to include the dimensional structure, different forms (alloy, oxide) and molecular catalysts in copper-based catalysts. Moreover, the reaction mechanisms …


Recent Advances In Bismuth-Based Co2 Reduction Electrocatalysts, Rui Zhou, Na Han, Yan-Guang Li Aug 2019

Recent Advances In Bismuth-Based Co2 Reduction Electrocatalysts, Rui Zhou, Na Han, Yan-Guang Li

Journal of Electrochemistry

Carbon dioxide (CO2) is an economical, secure and sustainable carbon resource around us. Its effective capture and recycling have been the focus of our entire society. Using the electrochemical method, CO2 can be reduced to different value-added chemicals or fuels. This approach not only would mitigate CO2 accumulation in the atmosphere, but also would help alleviate our dependence on fossil fuel. In this article, the basic principle and process of electrochemical CO2 reduction are first introduced. The recent development in bismuth-based catalysts for electrocatalytic CO2 reduction is reviewed with an emphasis on their preparation, …


Electrocatalytic Reduction Of Carbon Dioxide To Carbon Monoxide Using Cobalt Nitride, Chen Ma, Peng-Fei Hou, Peng Kang Aug 2019

Electrocatalytic Reduction Of Carbon Dioxide To Carbon Monoxide Using Cobalt Nitride, Chen Ma, Peng-Fei Hou, Peng Kang

Journal of Electrochemistry

Electrocatalytic reduction of carbon dioxide (CO2) is a promising method to alleviate global warming issues, although it still faces many challenges. Herein, we report cobalt nitride for electrocatalytic reduction of CO2 to carbon monoxide (CO) in an aqueous electrolyte. A comparison of catalysts with different preparation temperatures and atmospheres suggests that nitrogen doping is critical to improve catalytic activity. For the most active catalyst of 700-Co5.47N/C, the CO current density reached 9.78 mA·cm-2 at potential of -0.7 V vs. RHE. In addition, the CO/H2 ratio could be adjusted from 1:3 to 3:2 by …