Physical Sciences and Mathematics Commons^™

Design And Analysis For Melt Casting Metallic Fuel Pins Incorporating Volatile Actinides: Quarterly Progress Report 5/16/02- 8/15/02, Yitung Chen, Randy Clarksean, Darrell Pepper

Fuels Campaign (TRP)

An important aspect of the Advanced Accelerator Applications (AAA) program is the development of a casting process by which volatile actinide element (i.e., americium) can be incorporated into metallic alloy fuel pins. The traditional metal fuel casting process uses an inductively heated crucible.

This process works well for the fabrication of metal fuel pins traditionally composed of alloys of uranium and plutonium, but does not work well when highly volatile actinides are included in the melt. The problem occurs both during the extended time period required to superheat the alloy melt as well as when the chamber must be evacuated. …

Infrared Depletion Spectroscopy Of Aniline-Acetonitrile Cation And Aniline-Acetonitrile-Water Cation Clusters, H. Nagai, Naveed Piracha, T. Nakanaga

Naveed K. Piracha

The vibrational spectra of the aniline-acetonitrile^+ and the aniline-acetonitrile-water^+ cluster cations have been measured by the infrared depletion spectroscopy in the frequency region of NH and OH stretching vibrations. One absorption band was observed at 3437cm^-^1 in the infrared spectrum of the aniline-acetonitrile^+ cluster cation, and was assigned to the NH stretching vibration of free NH of aniline. As for the aniline-water-acetonitrile^+ cluster cation, three absorptions were observed at 3722, 3634 and 3247cm^-^1, which were assigned to the anti-symmetric stretching and symmetric stretching vibrations of OH of water and the stretching vibrations of NH bond interacting with water, respectively. In …

Maximization Of The Open Circuit Voltage For Hydrogenated Amorphous Silicon N–I–P Solar Cells By Incorporation Of Protocrystalline Silicon P-Type Layers, R. J. Koval, Chi Chen, G. M. Ferreira, A. S. Ferlauto, Joshua M. Pearce, P. I. Rovira, C. R. Wronski, R. W. Collins

Joshua M. Pearce

Scaling, Domains, And States In The Four-Dimensional Random Field Ising Magnet, Alan Middleton

Physics - All Scholarship

The four dimensional Gaussian random field Ising magnet is investigated numerically at zero temperature, using samples up to size $64^4$, to test scaling theories and to investigate the nature of domain walls and the thermodynamic limit. As the magnetization exponent $\beta$ is more easily distinguishable from zero in four dimensions than in three dimensions, these results provide a useful test of conventional scaling theories. Results are presented for the critical behavior of the heat capacity, magnetization, and stiffness. The fractal dimensions of the domain walls at criticality are estimated. A notable difference from three dimensions is the structure of the …

Magnetic Properties Of Nanoparticle Systems Of Fe, Co, Ni, And Fept, Created By Ion Implantation, Korey Dean Sorge

Doctoral Dissertations

Magnetization measurements have been performed on nanoparticle arrays of Fe, Co, Ni, and FePt in single-crystal substrates. Materials are formed by ion implantation into a layer followed by thermal annealing to give electrically isolated but crystallographically textured arrays. Studies show competition between effective single-particle anisotropy (due to magnetocrystalline, shape, surface, and stress effects) and macroscopic anisotropy due to dipolar interactions.

Results of these measurements are compared to expectations found in the well-known Stoner-Wohlfarth model of non-interacting, uniaxial particles. While this model is extensively used in magnetic materials research, the missing effects from dipolar interactions between particles give very different results …

Size And Structure Of The Narrow-Line Region Of Quasars, Nicola Bennert, Heino Falcke, Hartmut Schulz, Andrew S. Wilson, Beverley J. Wills

Physics

We have observed the narrow-line regions (NLRs) of the seven brightest radio-quiet Palomar-Green (or Bright Quasar Survey) quasars (z < 0.5) with the Wide Field Planetary Camera 2 on board the Hubble Space Telescope (HST). Linear-ramp filters were used to image the [O III] λ5007 line emission with 00455-01 pixel resolution. We find that the NLRs are very compact with typical extents of 2''-4''. Two quasars show compact filamentary structures similar to Seyfert NLRs. They may be related to radio outflows. Most interestingly, when including a sample of Seyfert galaxies observed with HST, we tentatively find that the size of the NLR is proportional to the square root …

Spin Injection Into Amorphous Semiconductors, Evgeny Y. Tsymbal, V. M. Burlakov, Ivan I. Oleinik

Evgeny Tsymbal Publications

Using a realistic model for the atomic and electronic structure of amorphous silicon, we explore spin injection into amorphous semiconductors. We calculate the spin-dependent conductance of magnetoresistive devices within the Landauer-Büttiker formalism including inelastic scattering. We find that reducing the density of injected carriers and increasing the spin polarization of the electrodes are favorable for spin injection, whereas inelastic scattering is detrimental, and show that the upper limit for magnetoresistance is given by Julliere's formula.

Competition Between Ferromagnetic Metallic And Paramagnetic Insulating Phases In Manganites, G. Li, H. D. Zhou, S. J. Feng, Xiaojuan Fan, X. G. Li, Z. D. Wang

Physics Faculty Research

La_0.67Ca_0.33Mn_1−xCu_xO₃(x=0 and 0.15) epitaxial thin films were grown on the (100) LaAlO₃ substrates, and the temperature dependence of their resistivity was measured in magnetic fields up to 12 T by a four-probe technique. We found that the competition between the ferromagnetic metallic (FM) and paramagnetic insulating (PI) phases plays an important role in the observed colossal magnetoresistance(CMR) effect. Based on a scenario that the doped manganites approximately consist of phase-separated FM and PI regions, a simple phenomenological model was proposed to describe the CMR effect. Using this model, we …

Construction And Testing Of A Low-Finesse Fabry-Perot Interferometer For Use In Atomic Spectroscopy, Nathan C. Moody

Student Works

I built a low-finesse confocal cavity with aluminum mirrors for use in the imaging of ultra-cold calcium ion plasmas. The confocal cavity provides stability at large mirror separations, a condition necessary for achieving both low finesse and narrow peak widths. Additionally, the finesse in the case of coherent input is effectively doubled compared to multi-mode resonance. The cavity was tested using a GaN diode laser input at 397nm. The transmission obtained indicated that the finesse of the cavity was slightly lower than the prediction based on measurements of the mirror reflectivities and the assumption of incoherent input.

Magnetism Of Co Nanocluster Films, Y. Qiang, R.F. Sabiryanov, Sitaram Jaswal, Yi Liu, H. Haberland, David J. Sellmyer

David Sellmyer Publications

A cluster-beam technique is used to produce nearly monodispersed nanoclusters of Co while independently varying their size and concentration. The Co clusters are embedded in Cu and SiO₂ to form films with cluster size varying from 300 to 9000 atoms and Co concentration varying from 10 to 50 vol %. The Co magnetization (M_s) increases with increasing cluster size and decreases with increasing Co concentration for a given cluster size but is always less than the bulk value. First-principles calculations are used to analyze the experimental data in terms of the local environment effects at the …

A New Type Of Particle Detector For Nuclear Scattering Experiments, Philip Ugorowski

Dissertations

A new detector was needed for counting recoil protons resulting from proton-proton (pp) elastic scattering during pion production experiments by the Polarized Internal Target Experiments (PINTEX) group at Indiana University Cyclotron Facility (IUCF). The previous silicon detectors were only usable forincoming protons up to 9 MeV, and a stopping power of at least 40 MeV was needed. In addition, the detector had to operate in nanotorr vacuum, and near strong varying magnetic fields, ruling out standard organic plastic scintillators and photomultiplier tubes. We needed to find the most suitable inorganic scintillator and another method of detecting the photons produced when …

Corrosion Of Steel By Lead Bismuth Eutectic: Quarterly Report For May-June-July 2002, John Farley

Transmutation Sciences Materials (TRP)

The goal of this project is to understand the basic science of corrosion in the steel/LBE system.

We are taking more data, typically using the newly installed X-ray Photoelectron Spectrometry (XPS) apparatus, and analyzing our existing data. Undergraduate students Denise Parsons and Julia Manzerova have helped a great deal in the analysis of the data. We can obtain the elemental composition as a function of position within the sample. This gives clues to the migration of materials, the composition of the protective oxide layer, and the basic science of the corrosion process. We found dramatic differences between the exposed and …

Dose Coefficient (Dc) Methodology Report, John P. Shanahan, Phillip W. Patton, Mark Rudin

Transmutation Sciences Physics (TRP)

The purpose of this report is to present the methodology developed to calculate internal and external dose coefficients for radionuclides produced in the spallation process. Much of the information regarding computer codes in this report comes from various technical manuals and professional papers. References are provided at the beginning of each section for documentation and for the user who requires more specific information. The report also includes the results of applying the methodology to determine dose coefficients for five radionuclides. This effort identified potential areas of concern that will need to be addressed when the methodology is used in the …

Poiseuille Advection Of Chemical Reaction Fronts, Boyd F. Edwards

All Physics Faculty Publications

Poiseuille flow between parallel plates alters the shapes and velocities of chemical reaction fronts. In the narrow-gap limit, the cubic reaction-diffusion-advection equation predicts a front-velocity correction equal to the gap-averaged fluid velocity ϵ. In the singular wide-gap limit, the correction equals the midgap fluid velocity 3ϵ/2 when the flow is in the direction of propagation of the reaction front, and equals zero for adverse flow of any amplitude for which the front has a midgap cusp. Stationary fronts are possible only for adverse flow and finite gaps. Experiments are suggested.

Double-Logarithmic Two-Loop Self-Energy Corrections To The Lamb Shift, Ulrich D. Jentschura, I. Nandori

Physics Faculty Research & Creative Works

Self-energy corrections involving logarithms of the parameter Z α can often be derived within a simplified approach, avoiding calculational difficulties typical of the problematic nonlogarithmic corrections (as customary in bound-state quantum electrodynamics, we denote by Z the nuclear charge number, and by α the fine-structure constant). For some logarithmic corrections, it is sufficient to consider internal properties of the electron characterized by form factors. We provide a detailed derivation of related self-energy “potentials” that give rise to the logarithmic corrections; these potentials are local in coordinate space. We focus on the double-logarithmic two-loop coefficient B₆₂ for P states and …

Electron Correlation Leading To Double-K-Shell Vacancy Production In Li-Like Ions Colliding With Helium, Ali Sami Alnaser

Dissertations

Single and double K-shell vacancies in Li-like ions colliding with neutral helium target have been investigated using high-resolution Auger projectile spectroscopy. Be⁺, B²⁺, C³⁺, and O⁵⁺ Li-like ions were produced and accelerated to intermediate-to-high collision velocities where perturbative models are expected to be valid, using the Tandem Van de Graaff accelerator at Western Michigan University. Double-K-shell vacancies in atomic systems or so-called “ hollow ions” can be induced by different mechanism in ion-atom collisions. For intermediate-to-high velocity collisions where the collision time is small, the projectile ion can interact with only one of …

Simulations Of The Instability Of The M = 1 Self-Shielding Diocotron Mode In Finite-Length Non-Neutral Plasmas, Grant W. Mason, Ross L. Spencer

Faculty Publications

The "self-shielding" m = 1 diocotron mode in Malmberg-Penning traps has been known for over a decade to be unstable for finite length non-neutral plasmas with hollow density profiles. Early theoretical efforts were unsuccessful in accounting for the exponential growth and/or the magnitude of the growth rate. Recent theoretical work has sought to resolve the discrepancy either as a consequence of the shape of the plasma ends or as a kinetic effect resulting from a modified distribution function as a consequence of the protocol used to form the hollow profiles in experiments. Both of these finite length mechanisms have been …

Simple, Compact Source For Low-Temperature Air Plasmas, D. P. Sheehan, J. Lawson, M. Sosa, R. A. Long

Physics and Biophysics: Faculty Scholarship

A simple, compact source of low-temperature, spatially and temporally uniform air plasma using a Telsa induction coil driver is described. The low-power ionization discharge plasma is localized (2 cm X 0.5 cm X 0.1 cm) and essentially free of arc channels. A Teflon coated rolling cylindrical electrode and dielectric coated ground plate are essential to the source’s operation and allow flat test samples to be readily exposed to the plasma. The plasma is a copious source of ozone and nitrogen oxides. Its effects on various microbes are discussed.

Single-Molecule Imaging With A Custom-Built Fluorescence Microscope, David Allan Ball

Masters Theses

An apparatus for single-molecule imaging was constructed and used to examine nanomolar solutions of Bodipy Texas Red in water. The illumination source for this microscope is a synchronously pumped dye laser operating at a wavelength of 585 nm. The beam can easily be switched to give total internal reflection or wide field epi-illumination excitation of the sample. The instrument also has the capability of being used for single-molecule detection by confocal epiillumination and for fluorescence correlation spectroscopy. Movies of single molecules were analyzed using custom software written in Matlab. Molecules stuck to the surface revealed fluctuations in intensity, or blinking, …

44th Rocky Mountain Conference On Analytical Chemistry

Rocky Mountain Conference on Magnetic Resonance

Final program, abstracts, and information about the 44th annual meeting of the Rocky Mountain Conference on Analytical Chemistry, co-endorsed by the Colorado Section of the American Chemical Society and the Society for Applied Spectroscopy. Held in Denver, Colorado, July 28 - August 1, 2002.

An All Optical Laser Wakefield Electron Injector, Donald Umstadter

Donald Umstadter Publications

The personnel who were supported by the grant included the P.I. (Prof. Umstadter), several research scientists (A. Maksimchuk and V. Yanovsky), a postdoc (P. Zhang) and several graduate and undergraduate students.
Although there were several setbacks in developing the novel laser technology required to produce a monoenergetic beam of electrons from an all-optical accelerator, several important steps were taken towards reaching that ultimate goal. The most important outcome of this project was that we demonstrated the principle of optical control of laser accelerators, namely, that one laser pulse could modify the properties (e.g., emittance and electron number) of an electron …

Search For New Physics In Photon-Lepton Events In Pp̅ Collisions At √S= 1.8 Tev, Darin Acosta, Kenneth A. Bloom, Collider Detector At Fermilab Collaboration

Kenneth Bloom Publications

We present the results of a search in pp̅ collisions at √s = 1.8 TeV for anomalous production of events containing a photon and a lepton ( e or μ), both with large transverse energy, using 86 pb^-1 of data collected with the Collider Detector at Fermilab during the 1994–1995 collider run at the Fermilab Tevatron. The presence of large missing transverse energy (E_T), additional photons, or additional leptons in these events is also analyzed. The results are consistent with standard model expectations, with the possible exception of photon-lepton events with large E_T, for …

Nolan-Pollak Type Cn Counters In The Vienna Aerosol Workshop, J. L. Gras, Josef Podzimek, T. C. O'Connor, K. H. Enderle

Physics Faculty Research & Creative Works

Three "standard" Nolan-Pollak (N-P) and modified N-P design condensation nucleus (CN) counters were included in the Vienna Workshop on Intercomparison of Condensation Nuclei and Aerosol Particle counters. These counters came from diverse backgrounds, namely programs in USA, Europe and Australia. In this work, principles of the operation and previous history of calibration of the N-P expansion counter are briefly reviewed and comparisons between the particular counters used in the workshop are presented and discussed. Counting agreement was found to be very good between the N-P counters, typically better than ± 12% for a range of aerosol sizes and compositions from …

Measurement Of High-Q 2 Charged Current Cross Sections In E - P Deep Inelastic Scattering At Hera, S. Chekanov, D. Krakauer, S. Magill, B. Musgrave, J. Repond, R. Yoshida, Margarita C. K. Mattingly, P. Antonioli, G. Bari, M. Basile, L. Bellagamba, D. Boscherini, A. Bruni, G. Bruni, G. Cara Romeo, L. Cifarelli, F. Cindolo, A. Contin, M. Corradi, S. De Pasquale, P. Giusti, G. Iacobucci, G. Levi, A. Margotti, R. Nania, F. Palmonari, A. Pesci, G. Sartorelli, A. Zichichi, G. Aghuzumtsyan, D. Bartsch

Faculty Publications

Cross sections for e - p charged current deep inelastic scattering have been measured at a centre-of-mass energy of 318 GeV with an integrated luminosity of 16.4 pb -1 using the ZEUS detector at HERA. Differential cross sections dσ/dQ 2, dσ/dx and dσ/dy are presented for Q 2 > 200 GeV 2. In addition, d 2σ/(dxdQ 2) was measured in the kinematic range 280 GeV 2 < Q 2 < 30 000 GeV 2 and 0.015 < × < 0.42. The predictions of the Standard Model agree well with the measured cross sections. The mass of the W boson, determined from a fit to dσ/dQ 2, is M W = 80.3±2.1(stat.) ± 1.2(syst.) ± 1.0(PDF) GeV. © 2002 Published by Elsevier Science B.V.

Location Of Pc 1–2 Waves Relative To The Magnetopause, R E. Denton, J Labelle, X Zhu

Dartmouth Scholarship

Spacecraft-borne and ground-based magnetome- ters frequently detect magnetospheric micropulsations in the period range 0.2–10s, termed Pc 1–2, and attributed to electromagnetic ion cyclotron waves driven by temperature anisotropy (T⊥ > T∥). Previous surveys of Pc 1 occur- rence locations have been limited to L ≤ 9. We present AMPTE/IRM observations of the distribution of Pc 1 waves out to the magnetopause, for a limited region of MLT = 10–14. The probability of wave occurrence Pwav is large (> 0.15) between L = 7–12, peaking at L = 8–10 (Pwav ∼ 0.25). When the L-value is normalized to the magnetopause position Lmp, …

Density Profile And Flow Of Miscible Fluid With Dissimilar Constituent Masses, Ras B. Pandey, D. Stauffer, R. Seyfarth, Luis A. Cueva, J.F. Gettrust, Warren Wood

Faculty Publications

A computer simulation model is used to study the density profile and flow of a miscible gaseous fluid mixture consisting of differing constituent masses (m(A) = m(B)/3) through an open matrix. The density profile is found to decay with the height proportional to exp(-m(A(B))h), consistent with the barometric height law. The flux density shows a power-law increase proportional to (p(c) - p)(a) with mu similar or equal to 2.3 at the porosity 1 - p above the pore percolation threshold 1 - p(c). (C) 2002 Elsevier Science B.V. All rights reserved.

Electronic Transport Through A Nuclear-Spin-Polarization-Induced Quantum Wire, Yuriy V. Pershin Dr, S. N. Shevchenko, I. D. Vagner, P. Wyder

Faculty Publications

Electron transport in a low-dimensional structure—the nuclear-spin-polarization-induced quantum wire is theoretically studied. In the proposed system the local nuclear-spin polarization creates the effective hyperfine field that confines the electrons with the spins opposite to the hyperfine field to the regions of maximal nuclear-spin polarization. The influence of the nuclear-spin relaxation and diffusion on the electron energy spectrum and on the conductance of the quantum wire is calculated and the experimental feasibility is discussed.

Electrical Conductivity And Thermopower Of Cu–Sio[Sub 2] Nanogranular Films., W. Chen, J. Lin, X. Zhang, H. Shin, Jeffrey Dyck, C. Uher

Jeffrey Dyck

We have measured the thermopower S and electrical conductivity σ in a series of Cu[sub x](SiO[sub 2])[sub 1-x] nanogranular films between 2 and 300 K with Cu volume fraction x varying from 0.43 up to 1.0. At low temperatures, disorder-enhanced electron-electron interaction effects dictate the behavior of σ. A crossover of the temperature dependence from σ∝ √T to σ∝ T[sup 1/3] is observed as x is lowered and the metal-insulator transition is approached. S is small, shows linear temperature dependence, and is rather insensitive to the change of x. Effects of annealing are also discussed.

Highly Anisotropic Crystal Growth And Thermoelectric Properties Of K2bi8_Xsbxse13 Solid Solutions: Band Gap Anomaly At Low X, Jeffrey S. Dyck, Theodora Kyratsi, Wei Chan, Duck-Young Chung, Ctirad Uher, Konstantinos Paraskevopoulos, Mercouri Kanatzidis

Jeffrey Dyck

The thermoelectric properties of solid solutions of the type B -K2Bi8_xSbxSe13 (0

Band Structure Of Strained Gd(0001) Films, I. N. Yakovkin, Takashi Komesu, Peter A. Dowben

Peter Dowben Publications

The electronic structure of strained and unstrained Gd(0001) surfaces has been studied both theoretically and experimentally with spin-polarized photoemission spectroscopy and spin-polarized inverse photoemission spectroscopy. Good agreement between calculated surface bands and surface-induced features of the spectra provides the basis for a more detailed explanation of the origin of the spin-polarized bands than was previously possible. It has been found that observed relaxation of the expansively strained in-plane crystal lattice constant, of Gd(0001) on Mo(112), significantly affects the electronic structure of the surface.