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Articles 31381 - 31410 of 36659

Full-Text Articles in Physical Sciences and Mathematics

Metastable States In Classical And Quantum Systems, Mark Makela, Samantha Parmley, Roger Yu Jul 1997

Metastable States In Classical And Quantum Systems, Mark Makela, Samantha Parmley, Roger Yu

All Faculty Scholarship for the College of the Sciences

The classical vibrational metastable states in a one-dimensional two-mass system are investigated experimentally and theoretically via the transmission of a coherent wave packet propagating through the system. The Fourier transform of the vibrational signal recorded in between the masses reveals resonant excitations by the coherent wave packet. The time-resolved spectrum indicates that the lifetime of a metastable state of higher frequency is longer than that of lower frequency, which is in contrast with the quantum mechanical double-barrier system. This study, which is easily accessible to physics majors, also demonstrates quantum resonant tunneling in a very simple classical way.

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High Resolution Oi (630 Nm) Image Measurements Of Fregion Depletion Drifts During The Guara Campaign, Michael J. Taylor, J. Labelle, J. A.H. Sobral Jul 1997

High Resolution Oi (630 Nm) Image Measurements Of Fregion Depletion Drifts During The Guara Campaign, Michael J. Taylor, J. Labelle, J. A.H. Sobral

All Physics Faculty Publications

A high performance, all‐sky, imaging system has provided data on the evolution and drift motions of F‐region depletions above the magnetic dip equator at Alcântara, Brazil, (2.3°S, 44.5°W). Monochromatic images of depletions in the OI(630 nm) nightglow were recorded on eight nights during 1‐16 October, 1994, as part of the Guará campaign. The drift motions of the depletions were typically 80–100 m/s eastward prior to local midnight and reduced to a minimum of ∼30–50 m/s in the morning hours, in accord with previous observations. However, on October 2–3 and 12–13 the depletions were observed to reverse direction for ∼60–90 min, …

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Small Angle Neutron Scattering From Nanodroplet Aerosols, Barbara Ellen Wyslouzil, Janice L. Cheung, Gerald Wilemski, Reinhard Strey Jul 1997

Small Angle Neutron Scattering From Nanodroplet Aerosols, Barbara Ellen Wyslouzil, Janice L. Cheung, Gerald Wilemski, Reinhard Strey

Physics Faculty Research & Creative Works

We report the first measurements of small angle neutron scattering from an aerosol. The aerosol was produced by expanding a D2O-N2 vapor mixture in a supersonic Laval nozzle. The neutron wavelength (0.5 nm) is less than the typical particle size, and we can therefore derive the average particle size (5-8 nm), number density (~1012 cm-3), and polydispersity of the size distribution directly from the experimental data rather than by inferring them from complex models of particle formation and growth. We also predict and observe a Doppler shift-induced anisotropy in the scattering pattern due to …

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Resonance Feature In Al- Photodetachment Below The Al(3S24S 2S) Threshold, B.J. Davies, C.W. Ingram, D.J. Larson, Chien-Nan Liu, Anthony F. Starace Jul 1997

Resonance Feature In Al- Photodetachment Below The Al(3S24S 2S) Threshold, B.J. Davies, C.W. Ingram, D.J. Larson, Chien-Nan Liu, Anthony F. Starace

Anthony F. Starace Publications

Photodetachment of Al-(3s23p23 3P) near the threshold of the first excited state of neutral aluminum has been studied both experimentally and theoretically. A 19-keV mass-resolved Al- beam was intersected by a frequency-doubled neodymium-doped yttrium aluminum garnet pumped dye-laser beam, and the fast atoms created by detachment processes were detected. Measurements just below the threshold of the first excited state, Al(3s24s2S), find a large resonance peak in the detachment signal. An eigenchannel R-matrix calculation generates a resonance structure that is qualitatively similar to the data and identifies the large resonance …

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Nondipole Resonant X-Ray-Raman Spectroscopy: Polarized Inelastic Scattering At The K Edge Of Cl2, J. D. Mills, J. A. Sheehy, T. A. Ferrett, S. H. Southworth, R. Mayer, Dennis W. Lindle, P. W. Langhoff Jul 1997

Nondipole Resonant X-Ray-Raman Spectroscopy: Polarized Inelastic Scattering At The K Edge Of Cl2, J. D. Mills, J. A. Sheehy, T. A. Ferrett, S. H. Southworth, R. Mayer, Dennis W. Lindle, P. W. Langhoff

Chemistry and Biochemistry Faculty Research

Experimental and theoretical studies are reported on the inelastic (Raman) scattering of wavelength-selected polarized x rays from the K edge of gas-phase chlorine molecules. The polarized emission spectra exhibit prominent nondipole features consequent of phase variations of the incident and emitted radiation over molecular dimensions, as predicted by the Kramers-Heisenberg scattering formalism. Issues pursuant to the detection of core-hole localization by resonant Raman scattering from homonuclear diatomic molecules are critically examined. [S0031-9007(97)03486-8]

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Semiclassical Formula For Oscillator Strengths In Atomic Spectra, V. Kondratovich, John B. Delos Jul 1997

Semiclassical Formula For Oscillator Strengths In Atomic Spectra, V. Kondratovich, John B. Delos

Arts & Sciences Articles

A simple semiclassical formula is given for the oscillator strengths of high Rydberg states of a hydrogen atom in an electric field. The oscillator strength of a state is proportional to the square of the function representing the quantum angular distribution of outgoing waves, evaluated at the classical angle of ejection from the atom that sends the electron into a semiclassically quantized eigentrajectory. The formula gives an interpretation of the envelopes of Stark manifolds in photoabsorption spectra; it is in good agreement with quantum calculations. The formula may also be used for other integrable or near-integrable systems.

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Closed-Orbit Theory And The Photodetachment Cross Section Of H- In Parallel Electric And Magnetic Fields, Aaron D. Peters, Charles Jaffé, J. B. Delos Jul 1997

Closed-Orbit Theory And The Photodetachment Cross Section Of H- In Parallel Electric And Magnetic Fields, Aaron D. Peters, Charles Jaffé, J. B. Delos

Arts & Sciences Articles

In this paper we obtain a simple analytic formula for the photodetachment cross section of H− in parallel electric and magnetic fields. The three-dimensional semiclassical approximation predicts oscillations in the spectrum and correlates these oscillations with closed classical orbits. The cylindrical symmetry of the Hamiltonian produces some interesting effects. In particular, at boundary energies the semiclassical approximation fails as a focused cusp approaches the origin.

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Quantum Manifestations Of Bifurcations Of Closed Orbits In The Photoabsorption Spectra Of Atoms In Electric Fields, J. Gao, John B. Delos Jul 1997

Quantum Manifestations Of Bifurcations Of Closed Orbits In The Photoabsorption Spectra Of Atoms In Electric Fields, J. Gao, John B. Delos

Arts & Sciences Articles

The methods developed in the preceding paper (paper II) are used to construct a wave function near a bifurcation of classical orbits of an atomic electron in an electric field. A formula for the recurrence strength near the bifurcation is derived and compared with experimental measurements.

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The Use Of Operator Regularization In The Computation Of Effective Field Theories, Jeffrey M. Hersh Jul 1997

The Use Of Operator Regularization In The Computation Of Effective Field Theories, Jeffrey M. Hersh

Physics Theses & Dissertations

Current methods of computing low-energy effective field theories while being accurate are extremely cumbersome co implement. Operator regularization provides a way to calculate any desired effective field theory avoiding the tediousness of previous methods. This technique is shown to be an effective method in explicitly calculating the 1/mheavy corrections that match an original full theory to its low-energy effective counterpart. This is demonstrated up to two loop order for the case of a charged two field θ{4}{4} theory as well as up to one loop order for the Higgs sector of the Minimal Supersymmetric Model. Additionally, the renormalization …

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Features Of The Photon Statistics Of Two Coupled Electromagnetic Field Modes Under The Conditions Of Strong Mode Coupling, Mikhail E. Veisman, Serguei Y. Kalmykov Jun 1997

Features Of The Photon Statistics Of Two Coupled Electromagnetic Field Modes Under The Conditions Of Strong Mode Coupling, Mikhail E. Veisman, Serguei Y. Kalmykov

Serge Youri Kalmykov

The probabilities of transitions between the Fock states of two electromagnetic field modes under the influence of coupling between modes of finite duration are investigated. It is shown that the transition probability is a strongly oscillating function of the mode numbers of the photons. Under conditions in which the coupling frequency exceeds the geometric mean of the mode frequencies (strong coupling), large numbers of photons are excited in the mode with the lower frequency. The excitation of a two-dimensional radiation field oscillator and the ‘‘red’’ symmetry of the transition probabilities can be attributed to instability of the classical two-dimensional oscillator …

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Study Of Laser Plasma Interactions In The Relativistic Regime, Donald Umstadter Jun 1997

Study Of Laser Plasma Interactions In The Relativistic Regime, Donald Umstadter

Donald Umstadter Publications

We discuss the first experimental demonstration of electron acceleration by a laser wakefield over distances greater than a Rayleigh range (or the distance a laser normally propagates in vacuum). A self-modulated laser wakefield plasma wave is shown to have a field gradient that exceeds that of an RF Iinac by four orders of magnitude (E ≥ 200 GV/m) and accelerates electrons with over l-nC of charge per bunch in a beam with space-charge-limited emittance (1 mm-mrad). Above a laser power threshold, a plasma channel, created by the intense ultrashort laser pulse (I~ 4 x 1018 W/cm2, …

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A Measurement Of The Michel Parameters In Leptonic Decays Of The Tau, R. Ammar, Kenneth A. Bloom, Cleo Collaboration Jun 1997

A Measurement Of The Michel Parameters In Leptonic Decays Of The Tau, R. Ammar, Kenneth A. Bloom, Cleo Collaboration

Kenneth Bloom Publications

We have measured the spectral shape Michel parameters ρ and η using leptonic decays of the τ, recorded by the CLEO II detector. Assuming e-μ universality in the vectorlike couplings, we find ρeμ = 0.735 ± 0.013 ± 0.008 and ηeμ = 20.015 ± 0.061 ± 0.062, where the first error is statistical and the second systematic. We also present measurements for the parameters for e and μ final states separately.

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Initial Polar Mfe Observation Of Substorm Signatures In The Polar Magnetosphere, H. Kawano, G. Le, C. T. Russell, G. Rostoker, T. Mukai, Harlan E. Spence Jun 1997

Initial Polar Mfe Observation Of Substorm Signatures In The Polar Magnetosphere, H. Kawano, G. Le, C. T. Russell, G. Rostoker, T. Mukai, Harlan E. Spence

Physics & Astronomy

This paper studies substorm influences in the polar magnetosphere using data from the POLAR magnetic field experiment (MFE). The POLAR spacecraft remains in the high altitude polar magnetosphere for extended periods around apogee. There it can stay at nearly constant altitude through all phases of a substorm, which was not possible on previous missions. We report such an event on March 28, 1996. Ground magnetometers monitored substorm activity, while the POLAR spacecraft, directly over the pole at (−0.8, −0.6, 8.5) RE in GSM coordinates, observed a corresponding perturbation in the total magnetic field strength. The total magnetic field first …

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First Polar And 1995-034 Observations Of The Midaltitude Cusp During A Persistent Northward Imf Condition, M. Grande, J. Fennell, S. Livi, B. Kellett, C. Perry, P. Anderson, J. Roeder, Harlan E. Spence, T. Fritz, B. Wilken Jun 1997

First Polar And 1995-034 Observations Of The Midaltitude Cusp During A Persistent Northward Imf Condition, M. Grande, J. Fennell, S. Livi, B. Kellett, C. Perry, P. Anderson, J. Roeder, Harlan E. Spence, T. Fritz, B. Wilken

Physics & Astronomy

We present the first observations by Polar and 1995-034 of the mid-altitude cusp. On May 29, 1996, the Polar and 1995-034 spacecraft crossed into an extended cusp region. The region was characterized by intense fluxes of solar wind like ions in the energy range 1–10 keV that had angular distributions that showed evidence of flows and trapping. The ion composition data are combined with energetic proton observations from Polar and plasma observations from 1995-034 and DMSP satellites to examine the spatial and temporal extent and plasma characteristics of the cusp during a persistent northward IMF condition. The composition data is …

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A New, Temporarily Confined Population In The Polar Cap During The August 27, 1996 Geomagnetic Field Distortion Period, Jiasheng Chen, Theodore A. Fritz, Robert B. Sheldon, Harlan E. Spence, Walther N. Spjeldvik, Joseph F. Fennell, Stefano Livi Jun 1997

A New, Temporarily Confined Population In The Polar Cap During The August 27, 1996 Geomagnetic Field Distortion Period, Jiasheng Chen, Theodore A. Fritz, Robert B. Sheldon, Harlan E. Spence, Walther N. Spjeldvik, Joseph F. Fennell, Stefano Livi

Physics & Astronomy

On August 27, 1996, a two-hour energetic heavy ion event (∼1 MeV) was detected at 8:25 UT at apogee (∼9 Re and an invariant latitude of ∼80°), by the Charge and Mass Magnetospheric Ion Composition Experiment onboard POLAR. The event, with a maximum spin averaged peak flux of ∼150 particles/(cm²-sr-s-MeV), showed three local peaks corresponding to three localized regions; the ion pitch angle distributions in the three regions were different from an isotropic distribution and different from each other. No comparable flux was observed by the WIND spacecraft. The appearance of lower energy He++ and O > +2 during the event …

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Calculation Of Electronic Coupling Matrix Elements For Ground And Excited State Electron Transfer Reactions: Comparison Of The Generalized Mulliken–Hush And Block Diagonalization Methods, Robert J. Cave, Marshall D. Newton Jun 1997

Calculation Of Electronic Coupling Matrix Elements For Ground And Excited State Electron Transfer Reactions: Comparison Of The Generalized Mulliken–Hush And Block Diagonalization Methods, Robert J. Cave, Marshall D. Newton

All HMC Faculty Publications and Research

Two independent methods are presented for the nonperturbative calculation of the electronic coupling matrix element (Hab) for electron transfer reactions using ab initio electronic structure theory. The first is based on the generalized Mulliken–Hush (GMH) model, a multistate generalization of the Mulliken Hush formalism for the electronic coupling. The second is based on the block diagonalization (BD) approach of Cederbaum, Domcke, and co-workers. Detailed quantitative comparisons of the two methods are carried out based on results for (a) several states of the system Zn2OH2+ and (b) the low-lying states of the benzene–Cl atom complex and its contact ion pair. Generally …

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On The Stark Broadening Parameters Of The Two Nii Spectral Lines Of The 3d-4f Transition, Vladimir Milosavljevic, Stevan Djenize Jun 1997

On The Stark Broadening Parameters Of The Two Nii Spectral Lines Of The 3d-4f Transition, Vladimir Milosavljevic, Stevan Djenize

Articles

Stark parameters (width and shift) of two singly ionized nitrogen spectral lines, that belong to 3d-4f transition have been measured in a linear pulsed, low pressure, arc discharge in the nitrogen-oxygen plasma at a 54000 K electron temperature and at a 2.8×10 23 m−3 electron density. The measured values have been compared to the existing experimental and calculated data

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A Surface-Emitting Vacuum-Deposited Organic Light Emitting Device, V. Bulovic, Peifang Tian, P. E. Burrows, M. R. Gokhale, S. R. Forrest, M. E. Thompson Jun 1997

A Surface-Emitting Vacuum-Deposited Organic Light Emitting Device, V. Bulovic, Peifang Tian, P. E. Burrows, M. R. Gokhale, S. R. Forrest, M. E. Thompson

Peifang Tian

We demonstrate a vacuum-deposited organic light emitting device which emits from its top surface through a transparent indium-tin-oxide anode. This device employs a novel protective cap layer which prevents damage to the organic layers during sputter deposition of the anode, while also improving hole injection. Mechanisms of current transport and carrier injection from the contacts are investigated. This device configuration allows for integration of organic light emitting devices with n-channel field effect transistors used in display active matrix backplanes.

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Charge Transfer Between Neutral Atoms And Highly Ionized Species: Implications For Iso Observations, Gary J. Ferland, K. T. Korista, D. A. Verner, A. Dalgarno Jun 1997

Charge Transfer Between Neutral Atoms And Highly Ionized Species: Implications For Iso Observations, Gary J. Ferland, K. T. Korista, D. A. Verner, A. Dalgarno

Physics and Astronomy Faculty Publications

We estimate rate coefficients for charge transfer between neutral hydrogen and helium and moderately to highly ionized heavy elements. Although charge transfer does not have much influence on hot collisionally ionized plasmas, its effects on photoionized plasmas can be profound. We present several photoionization models that illustrate the significant effect of charge transfer on the far-infrared lines detected by ISO.

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Degenerate Layer At Gan/Sapphire Interface: Influence On Hall-Effect Measurements, David C. Look, Richard J. Molnar Jun 1997

Degenerate Layer At Gan/Sapphire Interface: Influence On Hall-Effect Measurements, David C. Look, Richard J. Molnar

Physics Faculty Publications

Temperature-dependent Hall-effect measurements in hydride vapor phase epitaxial GaN grown on sapphire can be well fitted over the temperature range 10–400 K by assuming a thin, degenerate n-type region at the GaN/sapphire interface. This degenerate interfacial region dominates the electrical properties below 30 K, but also significantly affects those properties even at 400 K, and can cause a second, deeper donor to falsely appear in the analysis. However, by using a two-layer Hall model, the bulk mobility and carrier concentration can be accurately ascertained.

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Calibration Methodology And Multiple Tip Structure By Scanning Tunneling Microscopy., Michael Stephen Gossman Jun 1997

Calibration Methodology And Multiple Tip Structure By Scanning Tunneling Microscopy., Michael Stephen Gossman

Electronic Theses and Dissertations

The scanning tunneling microscope has been in commercial use just over a decade. Due to its Quantum Mechanical nature, experiments in this area have been widely publicized to the scientific community. The apparatus is steadily growing easier to use, though fundamental problems are still present. In the first chapter, an address is given on the modem theory of tunneling to rationalize the conclusions Physicists made long ago about this phenomenon. The expanded theory generalizes the mathematical motivation for attempting such unique experiments and serves as a lead-in for the major components of the apparatus. Many texts do not quantize what …

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Physical Conditions Of The Coronal Line Region In Seyfert Galaxies, Jason W. Ferguson, Kirk Korista, Gary J. Ferland Jun 1997

Physical Conditions Of The Coronal Line Region In Seyfert Galaxies, Jason W. Ferguson, Kirk Korista, Gary J. Ferland

Physics and Astronomy Faculty Publications

The launch of the Infrared Space Observatory and new atomic data have opened a window for the study of high-ionization gas in active galactic nuclei (AGNs). We present the results of a large number of photoionization simulations of the "coronal line" region in AGNs, employing new atomic data from the Opacity and Iron Projects. Our grid of line emission spans 8 orders of magnitude in gas density and 14 orders of magnitude in ionizing flux in an effort to identify the optimal conditions in which these lines form. We show that coronal lines form at distances from just outside the …

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An Improved Multi-Layer Fabrication Process For Yba2Cu3O7-X-Based Circuits, H.Q. Li, R.H. Ono, L.R. Vale, D.A. Rudman, Sy_Hwang Liou, W.H. Mallison Jun 1997

An Improved Multi-Layer Fabrication Process For Yba2Cu3O7-X-Based Circuits, H.Q. Li, R.H. Ono, L.R. Vale, D.A. Rudman, Sy_Hwang Liou, W.H. Mallison

Sy-Hwang Liou Publications

Improved via connections in structures of YBa2Cu3O7-x/SrTiO3/ YBa2Cu3O7-x (YBCO/STO/YBCO) multilayers have been made using a combined HF wet-etching and ion-milling process. The critical current density Jc of the via is as high as 2×106 A/cm2 at 76 K, and is dominated by edge contacts in the ab-plane, YBCO and Sr2AlNbO6 (SAN) multilayer test circuits were also made with this process. The 4° crossovers in a SAN test chip had a critical temperature Tc of 88 K and Jc …

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Localization And Transport Effects In The Disordered Materials, Vladislav Malyshkin Jun 1997

Localization And Transport Effects In The Disordered Materials, Vladislav Malyshkin

Dissertations

No abstract provided.

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Debye-Series Analysis Of The First-Order Rainbow Produced In Scattering Of A Diagonally Incident Plane Wave By A Circular Cylinder, James A. Lock, Charles L. Adler Jun 1997

Debye-Series Analysis Of The First-Order Rainbow Produced In Scattering Of A Diagonally Incident Plane Wave By A Circular Cylinder, James A. Lock, Charles L. Adler

Physics Faculty Publications

We derive the Debye-series expansion of the partial-wave scattering and interior amplitudes for the interaction of a diagonally incident beam of arbitrary profile with an infinitely long homogeneous dielectric circular cylinder. We then discuss the physical interpretation of the various terms of the series. We also consider the one-internal-reflection Debye-series terms for diagonal plane-wave incidence and examine the first-order rainbow extinction transition as a function of the tilt angle of the incident plane wave. We experimentally observe the first-order rainbow extinction transition and compare our observations with the Debye-series predictions. (C) 1997 Optical Society of America.

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Anharmonic Potentials In Supercooled Liquids: The Soft-Potential Model, Ulrich Zürcher, T. Keyes Jun 1997

Anharmonic Potentials In Supercooled Liquids: The Soft-Potential Model, Ulrich Zürcher, T. Keyes

Physics Faculty Publications

Instantaneous normal modes (INM) are the harmonic approximation to liquid dynamics. This is an extension of the phonon description of lattice dynamics, in which case Bloch's theorem shows that all modes are extended. Long-range order is destroyed in liquids and glasses, and the INM spectrum has contributions from both extended and localized modes. We use the soft-potential mode to describe localized modes. This model is a high-temperature extension of the standard two-level-system model for glasses. The equilibrium position of any atom in the liquid has only temporary character, and relaxation processes in the liquid are associated with particles hopping over …

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Kinetics And Spectroscopy Of Brno, Patrick E. Godfrey Jun 1997

Kinetics And Spectroscopy Of Brno, Patrick E. Godfrey

Theses and Dissertations

The infrared spectra and photochemistry of nitrosyl bromide, BrNO, are important to characterizing the performance of a recently demonstrated Br(2P1/2)-NO(v=2 → v=1) transfer laser pumped by photolysis of iodine molecules. This wavelength agile, mid-infrared laser may be a desirable source for remote sensing and infrared countermeasures missions. Nitrosyl bromide also plays a role in the destruction of stratospheric ozone. The kinetics of BrNO formation and destruction were examined using time-resolved photolysis techniques. The equilibrium constant for the dark reaction Br2 + 2NO (reversible reaction) 2BrNO was determined as Keq 168 ± 23 /atm and …

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Optimization Considerations For Adaptive Optics Digital Imagery Systems, Robert T. Brigantic Jun 1997

Optimization Considerations For Adaptive Optics Digital Imagery Systems, Robert T. Brigantic

Theses and Dissertations

This dissertation had three objectives. The first objective was to develop image quality metrics that characterize Adaptive Optics System (AOS) performance. The second objective was to delineate control settings that maximize AOS performance. The third objective was to identify and characterize trade-offs between fully and partially compensated adaptive. For the first objective, three candidate image quality metrics were considered: the Strehl ratio, a novel metric that modifies the Strehl ratio by integrating the modulus of the average system optical transfer function to a 'noise-effective-cutoff' frequency at which some specified image spectrum signal-to-noise-ratio level is attained, and the noise-effective-cutoff frequency. It …

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Symmetry Breaking In Crossed Magnetic And Electric Fields, C. Neumann, R. Ubert, S. Freund, Et Al., John B. Delos Jun 1997

Symmetry Breaking In Crossed Magnetic And Electric Fields, C. Neumann, R. Ubert, S. Freund, Et Al., John B. Delos

Arts & Sciences Articles

We present the first observations of cylindrical symmetry breaking in highly excited diamagnetic hydrogen with a small crossed electric field, and we give a semiclassical interpretation of this effect. As the small perpendicular electric field is added, the recurrence strengths of closed orbits decrease smoothly to a minimum, and revive again. This phenomenon, caused by interference among the electron waves that return to the nucleus, can be computed from the azimuthal dependence of the classical closed orbits.

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Breakdown Of The Independent Particle Approximation In High-Energy Photoionization, E. W. B. Dias, H. S. Chakraborty, P. C. Deshmukh, S. T. Manson, Oliver Hemmers, P. Glans, D. Hansen, H. Wang, S. B. Whitfield, Dennis W. Lindle, R. Wehlitz, Jon C. Levin, I. A. Sellin Jun 1997

Breakdown Of The Independent Particle Approximation In High-Energy Photoionization, E. W. B. Dias, H. S. Chakraborty, P. C. Deshmukh, S. T. Manson, Oliver Hemmers, P. Glans, D. Hansen, H. Wang, S. B. Whitfield, Dennis W. Lindle, R. Wehlitz, Jon C. Levin, I. A. Sellin

Environmental Studies Faculty Publications

The independent particle approximation is shown to break down for the photoionization of both inner and outer nℓ (ℓ>0) electrons of all atoms, at high enough energy, owing to interchannel interactions with the nearby ns photoionization channels. The effect is illustrated for Ne 2p in the 1 keV photon energy range through a comparison of theory and experiment. The implications for x-ray photoelectron spectroscopy of molecules and condensed matter are discussed.

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