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Physics Faculty Research & Creative Works

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Full-Text Articles in Physical Sciences and Mathematics

In Situ Observations Of Air Traffic Emission Signatures In The North Atlantic Flight Corridor, Hans Schlager, Paul Konopka, P. Schulte, U. Schumann, H. Ziereis, F. Arnold, M. Klemm, Donald E. Hagen, Philip D. Whitefield, J. Ovarlez May 1997

In Situ Observations Of Air Traffic Emission Signatures In The North Atlantic Flight Corridor, Hans Schlager, Paul Konopka, P. Schulte, U. Schumann, H. Ziereis, F. Arnold, M. Klemm, Donald E. Hagen, Philip D. Whitefield, J. Ovarlez

Physics Faculty Research & Creative Works

Focussed aircraft measurements have been carried out over the eastern North Atlantic to search for signals of air traffic emissions in the flight corridor region. Observations include NO, NO2, HNO3, SO2, O3, H2O, total condensation nuclei (CN), and meteorological parameters. A flight pattern with constant-altitude north-south legs across the major North Atlantic air traffic tracks was flown. Signatures of air traffic emissions were clearly detected for NOx, SO2, and CN with peak concentrations of 2 ppbv, 0.25 ppbv, and 500 cm-3, respectively, exceeding background …


Chaotic Behavior And Damage Spreading In The Glauber Ising Model: A Master Equation Approach, Thomas Vojta May 1997

Chaotic Behavior And Damage Spreading In The Glauber Ising Model: A Master Equation Approach, Thomas Vojta

Physics Faculty Research & Creative Works

We investigate the sensitivity of the time evolution of a kinetic Ising model with Glauber dynamics against the initial conditions. To do so we apply the "damage spreading" method, i.e., we study the simultaneous evolution of two identical systems subjected to the same thermal noise. We derive a master equation for the joint probability distribution of the two systems. We then solve this master equation within an effective-field approximation which goes beyond the usual mean-field approximation by retaining the fluctuations though in a quite simplistic manner. The resulting effective-field theory is applied to different physical situations. It is used to …


Studies Of V, Nb, Cr, And Zr Substituted 2:17 Compounds And Their Carbides Using Neutron Diffraction, H. Luo, Z. Hu, Muguo Chen, William B. Yelon, G. K. Marasinghe, Peter C. Ezekwenna, William Joseph James, W. C. Chang, S. H. Tsai Apr 1997

Studies Of V, Nb, Cr, And Zr Substituted 2:17 Compounds And Their Carbides Using Neutron Diffraction, H. Luo, Z. Hu, Muguo Chen, William B. Yelon, G. K. Marasinghe, Peter C. Ezekwenna, William Joseph James, W. C. Chang, S. H. Tsai

Physics Faculty Research & Creative Works

Samples of Nd2Fe17-xTxCy with T=V, Nb, Cr, and Zr were prepared by melting of the constituent elements including C and studied by neutron diffraction. Comparing with their uncarbided counterparts, we found that the substituents transfer, more or less, from the 6c site to the 18f and 18h sites with the introduction of C atoms. This behavior appears to relate to the electronegativities between the C atoms and the early transition series elements because the 18f and 18h sites are near neighbors of the interstitial C site. However, the C effects in the V. …


Nonanalytic Behavior Of The Spin Susceptibility In Clean Fermi Systems, Dietrich Belitz, Theodore R. Kirkpatrick, Thomas Vojta Apr 1997

Nonanalytic Behavior Of The Spin Susceptibility In Clean Fermi Systems, Dietrich Belitz, Theodore R. Kirkpatrick, Thomas Vojta

Physics Faculty Research & Creative Works

The wave vector and temperature-dependent static spin susceptibility, Xs(Q, T), of clean interacting Fermi systems is considered in dimensions 1 ≤ d ≤ 3. We show that at zero temperature Xs is a nonanalytic function of |Q|, with the leading nonanalyticity being |Q|d-1 for 1 < d < 3, and Q2ln|Q| for d = 3. For the homogeneous spin susceptibility we find a nonanalytic temperature dependence Td-1 for 1 < d < 3. We give qualitative mode-mode coupling arguments to that effect, and corroborate these arguments by a perturbative calculation to second order in the electron-electron interaction amplitude. The implications of this, in particular for itinerant ferromagnetism, are discussed. We also point out the relation between our findings and established perturbative results for one-dimensional systems, as well as for the temperature dependence of Xs(Q = 0) in d = 3.


Monte Carlo Simulations Of The Dynamical Behavior Of The Coulomb Glass, Torsten Wappler, Thomas Vojta, Michael Schreiber Mar 1997

Monte Carlo Simulations Of The Dynamical Behavior Of The Coulomb Glass, Torsten Wappler, Thomas Vojta, Michael Schreiber

Physics Faculty Research & Creative Works

We study the dynamical behavior of disordered many-particle systems with long-range Coulomb interactions by means of damage-spreading simulations. In this type of Monte Carlo simulation one investigates the time evolution of the damage, i.e., the difference of the occupation numbers of two systems, subjected to the same thermal noise. We analyze the dependence of the damage on temperature and disorder strength. For zero disorder the spreading transition coincides with the equilibrium phase transition, whereas for finite disorder we find evidence for a dynamical phase transition well below the transition temperature of the pure system.


Projectile Charge-State Dependence On Final-State Momentum Distributions For Single Ionization Of Helium, C. J. Wood, C. R. Feeler, Ronald E. Olson Jan 1997

Projectile Charge-State Dependence On Final-State Momentum Distributions For Single Ionization Of Helium, C. J. Wood, C. R. Feeler, Ronald E. Olson

Physics Faculty Research & Creative Works

Single-ionization cross sections and final-state momentum distributions have been calculated for the single-ionization collision reactions H[Formula Presented], [Formula Presented], He[Formula Presented], C[Formula Presented], and C[Formula Presented] + He at 100 keV/u. The classical trajectory Monte Carlo method has been used with a Wigner distribution to improve both the He electron classical radial and momentum distributions. Final-state ionized electron momenta are projected into a collision plane defined by the initial projectile momentum and the final transverse component of the He[Formula Presented] recoil momentum, with the results displayed differentially in various components of electron and recoil momenta. Positively charged projectile impact shows …


Momentum Spectra For Single And Double Electron Ionization Of He In Relativistic Collisions, C. J. Wood, Ronald E. Olson, W. Schmitt, R. Moshammer, J. Ullrich Jan 1997

Momentum Spectra For Single And Double Electron Ionization Of He In Relativistic Collisions, C. J. Wood, Ronald E. Olson, W. Schmitt, R. Moshammer, J. Ullrich

Physics Faculty Research & Creative Works

The complete momentum spectra for single and double ionization of He by [Formula Presented] [Formula Presented] [Formula Presented] have been investigated using a classical trajectory Monte Carlo method corrected for the relativistic projectile. The [Formula Presented] electron-electron interaction has been included in the post-collision region for double ionization to incorporate the effects of both the nuclear-electron and electron-electron ionizing interactions, and to access the effects of electron correlation in the electron spectra. Experimental measurements were able to determine the longitudinal momentum spectra for single ionization; these observations are in accordance with the theoretical predictions for the three-body momentum balance between …


Complete Momentum Balance For Single Ionization Of Helium By Fast Ion Impact: Experiment, R. Moshammer, J. Ullrich, H. Kollmus, W. Schmitt, M. Unverzagt, H. Schmidt-Böcking, C. J. Wood, Ronald E. Olson Jan 1997

Complete Momentum Balance For Single Ionization Of Helium By Fast Ion Impact: Experiment, R. Moshammer, J. Ullrich, H. Kollmus, W. Schmitt, M. Unverzagt, H. Schmidt-Böcking, C. J. Wood, Ronald E. Olson

Physics Faculty Research & Creative Works

The collision dynamics of He single ionization by [Formula Presented] impact was explored using the reaction microscope of the Gesellschaft für Schwerionenforschung, a high-resolution integrated multielectron recoil-ion momentum spectrometer. The complete three-particle final-state momentum distribution (nine Cartesian components [Formula Presented]) was imaged with a resolution of [Formula Presented] by measuring the three momentum components of the emitted electron and the recoiling target ion in coincidence. The projectile energy loss has been determined on a level of [Formula Presented] and projectile scattering angles as small as [Formula Presented] became accessible. The experimental data which are compared with results of classical trajectory …


Observation Of Upper Tropospheric Sulfur Dioxide- And Acetone-Pollution: Potential Implications For Hydroxyl Radical And Aerosol Formation, F. Arnold, J. Schneider, K. Gollinger, H. Schlager, P. Schulte, Donald E. Hagen, Philip D. Whitefield, Peter F. J. Van Velthoven Jan 1997

Observation Of Upper Tropospheric Sulfur Dioxide- And Acetone-Pollution: Potential Implications For Hydroxyl Radical And Aerosol Formation, F. Arnold, J. Schneider, K. Gollinger, H. Schlager, P. Schulte, Donald E. Hagen, Philip D. Whitefield, Peter F. J. Van Velthoven

Physics Faculty Research & Creative Works

Aircraft-based measurements of sulfur dioxide, acetone, carbon dioxide, and condensation nuclei (CN) were made over the north-eastern Atlantic at upper tropospheric altitudes, around 9000 m. On October 14, 1993, strong SO 2- and acetone-pollution (both up to 3 ppbv) were observed, which were accompanied by a CO 2-enhancement of up to 6 ppmv, and large CN-concentrations of up to about 1500 cm -3 (for radii ≥ 6 nm). CN, excess CO 2, and to a lesser degree also acetone, were positively correlated with SO 2. Air mass trajectory analyses indicate, that most of the air masses …


Ionization Of Helium In The Attosecond Equivalent Light Pulse Of 1 Gev/Nucleon U⁹²⁺ Projectiles, R. Moshammer, W. Schmitt, J. Ullrich, H. Kollmus, A. Cassimi, R. Dörner, O. Jagutzki, R. Mann, Ronald E. Olson, H. T. Prinz, H. Schmidt-Böcking, L. Spielberger Jan 1997

Ionization Of Helium In The Attosecond Equivalent Light Pulse Of 1 Gev/Nucleon U⁹²⁺ Projectiles, R. Moshammer, W. Schmitt, J. Ullrich, H. Kollmus, A. Cassimi, R. Dörner, O. Jagutzki, R. Mann, Ronald E. Olson, H. T. Prinz, H. Schmidt-Böcking, L. Spielberger

Physics Faculty Research & Creative Works

Single and double ionization of helium by 1 GeV/nucleon U92+ impact was explored in a kinematically complete experiment. The relativistic ion generates a subattosecond (10−18s) superintense (I > 1019W/cm2) electromagnetic pulse, which is interpreted as a field of equivalent photons (Weizsäcker-Williams method). Cross sections, the emission characteristics of ions and electrons as well as momentum balances, are quantitatively discussed in terms of photoionization of the atom in this broadband, ultrashort virtual photon field. © 1997 The American Physical Society.


Droplet Concentration And Size Distribution In Haze And Fog, Josef Podzimek Jan 1997

Droplet Concentration And Size Distribution In Haze And Fog, Josef Podzimek

Physics Faculty Research & Creative Works

Fog (haze) droplet concentrations and size distributions were measured at five sampling sites representing rural and urban regions and a highly polluted marine-urban environment. Droplet imprints in a thin gelatine layer were evaluated and compared to the measurement by light scattering instruments. This enabled conditions for the application of the logarithmic-normal size distribution and for the classification of typical fog droplet size distributions to be established. In particular, the parameters featuring the width and asymmetry of a size distribution were suggested and calculated. Advantages and drawbacks of the applied droplet sampling and evaluation technique are discussed in more detail. © …


Velocity Space "Snapshots" Of Continuum Electrons Produced By Slow, Bare, Highly Charged Ions: Saddle-Point Electrons?, M. Abdallah, S. Kravis, C. L. Cocke, Y. D. Wang, M. Stöckli, Ronald E. Olson Jan 1997

Velocity Space "Snapshots" Of Continuum Electrons Produced By Slow, Bare, Highly Charged Ions: Saddle-Point Electrons?, M. Abdallah, S. Kravis, C. L. Cocke, Y. D. Wang, M. Stöckli, Ronald E. Olson

Physics Faculty Research & Creative Works

Comprehensive velocity-space "snapshots" of the electron continua produced by the impact of ions on He at a projectile velocity of 1.63 a.u. have been measured for the bare projectiles of p, He, C, O and Ne. For the three highly charged ions, this velocity lies in the "ionization threshold" region where electron capture dominates the reaction. The experimental technique projects the distribution of soft continuum electrons onto a two-dimensional detector in such a way that the velocity-space distribution for all electrons with laboratory energies in the range from 0-30eV is accurately imaged. The data show no evidence for a saddle-point …


Three-Body Models Of Electron-Hydrogen Ionization, Stephenie J. Jones, Don H. Madison, Dmitry A. Konovalov Jan 1997

Three-Body Models Of Electron-Hydrogen Ionization, Stephenie J. Jones, Don H. Madison, Dmitry A. Konovalov

Physics Faculty Research & Creative Works

In this paper, we report calculations of electron-hydrogen ionization whereby the final-state wave Function is approximated by recently reported analytical three-body wave functions. In a first model we use the wave function of Alt and Mukhamedzhanov [Phys. Rev. A 47, 2004 (1993)], and in a second model we use the wave function of Berakdar [Phys. Rev. A 53, 2314 (1996)].


The Interaction Of Fast Alpha Particles With Pellet Ablation Clouds, J. M. Mcchesney, P. B. Parks, R. K. Fisher, Ronald E. Olson Jan 1997

The Interaction Of Fast Alpha Particles With Pellet Ablation Clouds, J. M. Mcchesney, P. B. Parks, R. K. Fisher, Ronald E. Olson

Physics Faculty Research & Creative Works

The energy spectra of energetic confined alpha particles are being measured using the pellet charge exchange method [R. K. Fisher, J. S. Leffler, A. M. Howald, and P. B. Parks, Fusion Technol. 13, 536 (1988)]. The technique uses the dense ablation cloud surrounding an injected impurity pellet to neutralize a fraction of the incident alpha particles, allowing them to escape from the plasma where their energy spectrum can be measured using a neutral particle analyzer. The signal calculations given in the above-mentioned reference disregarded the effects of the alpha particles' helical Larmor orbits, which causes the alphas to make multiple …


Semiquantal Modeling Of Thermal Vibrational Relaxation Of Diatomic Molecules, Ronald James Bieniek, Steven J. Lipson Dec 1996

Semiquantal Modeling Of Thermal Vibrational Relaxation Of Diatomic Molecules, Ronald James Bieniek, Steven J. Lipson

Physics Faculty Research & Creative Works

Vibrationally excited molecules play an important role in the spectroscopy, energetics, and chemical behavior of a wide range of gaseous systems of scientific and applied interest. Unfortunately, many desired collisional relaxation rates have not yet been experimentally measured, and current theoretical methods are often inadequate or too cumbersome for practical application. We report a semiquantal two-parameter scaling method for predicting relaxation rates that is very simple to employ, and impressively fits the temperature and vibrational dependencies of quantum mechanical and experimental collisional relaxation rates for several diatomic molecules (e.g., N2, HF, OH, NO) over many orders of magnitude.


Angle-Resolved X-Ray Circular And Magnetic Circular Dichroisms: Definitions And Applications, Sy Y. Tong, X. Q. Guo, James G. Tobin, George Daniel Waddill Dec 1996

Angle-Resolved X-Ray Circular And Magnetic Circular Dichroisms: Definitions And Applications, Sy Y. Tong, X. Q. Guo, James G. Tobin, George Daniel Waddill

Physics Faculty Research & Creative Works

We introduce definitions of angle-resolved x-ray circular dichroism (ARXCD) and magnetic x-ray circular dichroism (ARMXCD). As defined, the much larger effect of circular dichroism (ARXCD) is separated from the smaller magnetic (ARMXCD) effect. In all materials, ARXCD is zero along mirror planes while nonzero elsewhere. ARMXCD is nonzero only in magnetic materials. The measurement and analysis of ARMXCD allow element specific surface magnetism and surface structure as well as their inter-relationship to be studied as functions of the outgoing electron's direction.


Breakdown Of Landau-Ginzburg-Wilson Theory For Certain Quantum Phase Transitions, Thomas Vojta, Dietrich Belitz, Rajesh S. Narayanan, Theodore R. Kirkpatrick Oct 1996

Breakdown Of Landau-Ginzburg-Wilson Theory For Certain Quantum Phase Transitions, Thomas Vojta, Dietrich Belitz, Rajesh S. Narayanan, Theodore R. Kirkpatrick

Physics Faculty Research & Creative Works

The quantum ferromagnetic transition of itinerant electrons is considered. It is shown that the Landau-Ginzburg-Wilson theory described by Hertz and others breaks down due to a singular coupling between fluctuations of the conserved order parameter. This coupling induces an effective long-range interaction between the spins of the form 1/r2d-1. It leads to unusual scaling behavior at the quantum critical point in 1 < d ≤ 3 dimensions, which is determined exactly.


Theory Of The Seebeck Coefficient In Lacro₃ And Related Perovskite Systems, D. B. Marsh, Paul Ernest Parris Sep 1996

Theory Of The Seebeck Coefficient In Lacro₃ And Related Perovskite Systems, D. B. Marsh, Paul Ernest Parris

Physics Faculty Research & Creative Works

We consider the Seebeck coefficient in LaCrO3 and related transition-metal-oxide perovskites using a model for electronic conduction based on the electronic structure of the 3d orbitals of the B-site transition-metal cations. Relations for the Seebeck coefficient are presented for those perovskite systems in which electronic conduction is through the t2g states of the B-site transition-metal cations. High- and low-temperature limits for the Seebeck coefficient are identified for the cases of both strong and weak magnetic coupling between electron spins. In these high- and low-temperature limits, the Seebeck coefficient is determined as a function of carrier concentration. Results are …


Higher-Order Binding Corrections To The Lamb Shift Of 2p States, Ulrich D. Jentschura, Krzysztof Pachucki Sep 1996

Higher-Order Binding Corrections To The Lamb Shift Of 2p States, Ulrich D. Jentschura, Krzysztof Pachucki

Physics Faculty Research & Creative Works

We present an improved calculation of higher-order corrections to the one-loop self-energy of 2P states in hydrogenlike systems with small nuclear charge Z. The method is based on a division of the integration with respect to the photon energy into a high- and a low-energy part. The high-energy part is calculated by an expansion of the electron propagator in powers of the Coulomb field. The low-energy part is simplified by the application of a Foldy-Wouthuysen transformation. This transformation leads to a clear separation of the leading contribution from the relativistic corrections and removes higher-order terms. The method is applied to …


Relation Between Charge-Dipole Interactions And The Sqrt(E)-Dependent Mobility In Molecularly Doped Polymers, Paul Ernest Parris Aug 1996

Relation Between Charge-Dipole Interactions And The Sqrt(E)-Dependent Mobility In Molecularly Doped Polymers, Paul Ernest Parris

Physics Faculty Research & Creative Works

Time-of-flight measurements on a wide variety of molecularly-doped polymers reveal carrier mobilities that exhibit an exponential dependence on the square root of the applied electric field. Recent attempts to explain the observed field dependence have focused on the role played by spatial and energetic disorder. It as also been conjectured that the charge-dipole interactions often identified as the source of energetic disorder could be of sufficient range to lead to correlations in the energies of neighboring hopping sites. We have analytically explored the effect of such correlations on high field carrier transport in random potentials, and discuss how particular features …


Neutron Diffraction Structural Study Of Ce₂Fe₁₇₋ₓgaₓ, H. Luo, Z. Hu, William B. Yelon, Sanjay R. Mishra, Gary J. Long, Oran Allan Pringle, D. P. Middleton, K. H. J. Buschow Aug 1996

Neutron Diffraction Structural Study Of Ce₂Fe₁₇₋ₓgaₓ, H. Luo, Z. Hu, William B. Yelon, Sanjay R. Mishra, Gary J. Long, Oran Allan Pringle, D. P. Middleton, K. H. J. Buschow

Physics Faculty Research & Creative Works

Six samples of Ce2Fe17-xGax with nominal Ga content x equal to 0, 0.3, 0.5, 0.7, 1.0, 2.0 have been studied by powder neutron diffraction at room temperature. Both crystalline and magnetic refinements have been carried out. All six samples adopt the Th2Zn17-type rhombohedral structure. The only additional phase found is α-iron. Gallium atoms are found to have high affinity for the iron 18h site, and are absent from the 9d and 18f sites. The Ga substitution for Fe leads to an expansion of both the a and c axes. The Curie …


Anisotropy And Polarization In Charge Changing Collisions Of C⁴⁺ With Na(3s) And Laser Aligned Na(3p), S. Schippers, R. Hoekstra, R. Morgenstern, Ronald E. Olson Jul 1996

Anisotropy And Polarization In Charge Changing Collisions Of C⁴⁺ With Na(3s) And Laser Aligned Na(3p), S. Schippers, R. Hoekstra, R. Morgenstern, Ronald E. Olson

Physics Faculty Research & Creative Works

Absolute cross sections for C3+(6→5) emission at 465.7 nm after collisions of C4+ ions with ground state Na(3s) and laser excited aligned Na(3p) atoms are measured over the collision energy range of 3-7 keV amu-1. For Na(3s) polarizations are observed by measuring the linear polarization of the emitted light. In these collisions the polarization is found to be 0.33 and almost independent of the collision energy. Cross sections for collisions with the Na(3p) target are up to five times larger than for collisions with Na(3s). Slightly larger cross sections are measured when the laser excited Na(3p) target is Π-aligned as …


Binary Nucleation Kinetics. Iii. Transient Behavior And Time Lags, Barbara Ellen Wyslouzil, Gerald Wilemski Jul 1996

Binary Nucleation Kinetics. Iii. Transient Behavior And Time Lags, Barbara Ellen Wyslouzil, Gerald Wilemski

Physics Faculty Research & Creative Works

Transient binary nucleation is more complex than unary because of the bidimensionality of the cluster formation kinetics. To investigate this problem qualitatively and quantitatively, we numerically solved the birth-death equations for vapor-to-liquid phase transitions. Our previous work [J. Chem. Phys 103, 1137 (1995)] showed that the customary saddle point and growth path approximations are almost always valid in steady state gas phase nucleation and only fail if the nucleated solution phase is significantly nonideal. The current work demonstrates that in its early transient stages, binary nucleation rarely, if ever, occurs via the saddle point. This affects not only the number …


Charge-Dipole Model For The Universal Field Dependence Of Mobilities In Molecularly Doped Polymers, David H. Dunlap, Paul Ernest Parris, Vasudev M. Kenkre Jul 1996

Charge-Dipole Model For The Universal Field Dependence Of Mobilities In Molecularly Doped Polymers, David H. Dunlap, Paul Ernest Parris, Vasudev M. Kenkre

Physics Faculty Research & Creative Works

Using the general result that the mobility μ, of charge carriers driven in a spatially correlated random potential by an electric field E can be expressed in terms of the Laplace transform of a particular correlation function related to the random potential, we demonstrate that the exponential dependence of μ on √E universally observed in molecularly doped polymers arises naturally from the interaction of charge carriers with randomly distributed permanent dipoles.


Structural And Magnetic Studies On Prba2fe3o8, V. P.S. Awana, Latika Menon, S. K. Malik, Apurva Mehta, Sanjay Mishra, William B. Yelon Jun 1996

Structural And Magnetic Studies On Prba2fe3o8, V. P.S. Awana, Latika Menon, S. K. Malik, Apurva Mehta, Sanjay Mishra, William B. Yelon

Physics Faculty Research & Creative Works

It is known that Fe moments order antiferromagnetically with Néel temperature, TN, above 700 K in RBa2Fe3O7-δ with R=Y and Eu, and Pr moments order antiferromagnetically in PrBa2Cu3,O7-δ, with TN of 17 K. We have synthesized PrBa2Fe3O8 to study the ordering of Pr and Fe moments. From X-ray and neutron diffraction studies, this compound is found to crystallize in the tetragonal structure (space group P4/mmm). 57Fe Mössbauer studies show a complex hyperfine split pattern at 77 K, but a doublet superimposed on a six-line pattern at 300 K implying that some of the Fe moments order magnetically between 77 and …


A Classical Analysis Of Proton Collisions With Ground-State And Excited, Aligned Sodium Targets, C. J. Lundy, Ronald E. Olson May 1996

A Classical Analysis Of Proton Collisions With Ground-State And Excited, Aligned Sodium Targets, C. J. Lundy, Ronald E. Olson

Physics Faculty Research & Creative Works

The dependence of electron capture and ionization processes on the pre-collision electronic distribution is examined for the systems H+ + Na(3s, 3pΣ, 3pΠ) primarily in the energy range 1-15 keV. Populations of the capture and ionization channels as well as the coherence of the post-collision electronic distribution of the capture product are formulated using the classical trajectory Monte Carlo (CTMC) method. Total capture and ionization cross sections arising from initially aligned Na(3p) targets exhibit transient behaviour near the velocity-matching energy of 5.7 keV. This observation is described in terms of anisotropy parameters; anisotropy effects are also analysed for the capture …


State-Selective Electron Capture In Low Velocity Multiply Charged Ion, Helium Collisions, A. Cassimi, S. Duponchel, X. Flechard, P. Jardin, P. Sortais, D. Hennecart, Ronald E. Olson May 1996

State-Selective Electron Capture In Low Velocity Multiply Charged Ion, Helium Collisions, A. Cassimi, S. Duponchel, X. Flechard, P. Jardin, P. Sortais, D. Hennecart, Ronald E. Olson

Physics Faculty Research & Creative Works

Recoil ion momentum spectroscopy has been applied to study low energy, state-selective single electron capture by highly charged projectiles. The specific systems investigated are fully stripped 6.82 keV/u Ne10+ 6.82 keV/u Ar18+ on He. Measurements of the He+ recoil ion longitudinal momenta are used to determine the final n-state dependence of the captured electron. Simultaneous measurement of the transverse momenta of the recoil ion yields information about the impact parameter dependence of the reaction and the reaction window for electron capture. © 1996 The American Physical Society.


Site Affinity Of Substituents In Nd₂Fe₁₇₋ₓtₓ (T=Cu,Zr,Nb,Ti,V) Alloys, William B. Yelon, Z. Hu, William Joseph James, G. K. Marasinghe Apr 1996

Site Affinity Of Substituents In Nd₂Fe₁₇₋ₓtₓ (T=Cu,Zr,Nb,Ti,V) Alloys, William B. Yelon, Z. Hu, William Joseph James, G. K. Marasinghe

Physics Faculty Research & Creative Works

In order to understand the magnetic properties of the substituted rare-earth-iron alloys, it is especially important to know the location of the substitutional atoms within the iron lattice. The site distributions of some nontransition-metal substituents in the substituted Nd2Fe17-xTx alloys have previously been reported. Here we report the site distributions of some transition-metal substituents (Cu,Zr,Nb,Ti,V) in the Nd2Fe17-xTx alloys and compare them with those of the nontransition-metal substituted compounds. Rietveld analysis of neutron powder diffraction data indicates that the nontransition-metal substituents show very similar site affinity at low substituent content. …


Neutron Diffraction And Magnetic Studies Of Rfe₁₂₋ₓtₓcY (R=Y,Er; T=V,Ti,Mo) Alloys, Z. Hu, William B. Yelon, X. D. Zhang, William Joseph James Apr 1996

Neutron Diffraction And Magnetic Studies Of Rfe₁₂₋ₓtₓcY (R=Y,Er; T=V,Ti,Mo) Alloys, Z. Hu, William B. Yelon, X. D. Zhang, William Joseph James

Physics Faculty Research & Creative Works

RFe12-xTxCy, (R=Y,Er; T=V,Ti,Mo) alloys were prepared by rf induction melting and analyzed using neutron powder diffraction and superconducting quantum interference device (SQUID) measurements. Rietveld analysis of the neutron diffraction data indicates that V, Ti, and Mo atoms all prefer the 8i sites. The refined amount of carbon atoms found in the interstitial sites from neutron diffraction data is significantly less than the nominal carbon content. All samples have the easy direction along the c axis. The Er sublattice couples to the Fe sublattice antiferromagnetically. The average Fe site moments range from 1.3 to 2.8 …


Neutron Diffraction Studies Of Ndₙfeₘ₋ₓ₋YVₓalY [(N,M)=(1,12), (2,17), (3,29)], Z. Hu, William B. Yelon, William Joseph James Apr 1996

Neutron Diffraction Studies Of Ndₙfeₘ₋ₓ₋YVₓalY [(N,M)=(1,12), (2,17), (3,29)], Z. Hu, William B. Yelon, William Joseph James

Physics Faculty Research & Creative Works

Several NdnFem-x-yVxAly [(n,m)=(1,12), (2,17), (3,29)] samples were prepared and analyzed using neutron powder diffraction. Rietveld analysis of the neutron diffraction data indicates that the V and Al substituents take those sites with similar environments in all three phases, as observed in our previous study of Ti-substituted compounds. It was confirmed that the diffraction data of the 3:29 compound can be better refined using the A2/m space group than using the P21/c space group. The SQUID measurements show that all samples have Curie temperatures well above room temperature. The neutron diffraction results …