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2020

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Articles 14311 - 14340 of 15207

Full-Text Articles in Physical Sciences and Mathematics

Discriminative Factorization Models For Student Behavioral Pattern Detection And Classification, Mehrdad Mirzaei Jan 2020

Discriminative Factorization Models For Student Behavioral Pattern Detection And Classification, Mehrdad Mirzaei

Legacy Theses & Dissertations (2009 - 2024)

The goal of this dissertation is to examine factors such as how a student chooses to engage with the online platform and time spent on individual tasks and draw conclusions to improve the efficiency of the students and efficacy of online learning tools. Student activities and decision-making while functioning in a computer-based learning environment are utilized to guide students with effective patterns in studying. In addition to the sequence of actions, we have considered the time spent on each activity in modeling to have a more accurate representation of students' behavior in studying. Using sequential pattern mining methods, we find …


Units Of Truncated Group Rings Of Higman Groups, Brian Rich Jan 2020

Units Of Truncated Group Rings Of Higman Groups, Brian Rich

Legacy Theses & Dissertations (2009 - 2024)

In this thesis an analogue of the triviality of units of group rings of finite abelian groupsis proved for truncated group rings. A Higman group is a group of exponent 2, 3, 4 or 6. The truncated group ring ZG t is the quotient of the group ring by the ideal generated by the formal sum of all group elements. We show that in the case of finite abelian G that ZG t has only trivial units; i.e, that any unit in ZG t is an image under the quotient map of a unit of the form ±g, where g …


Towards Practical Modulation Recognition For Future Spectrum-Sharing Applications, Wei Xiong Jan 2020

Towards Practical Modulation Recognition For Future Spectrum-Sharing Applications, Wei Xiong

Legacy Theses & Dissertations (2009 - 2024)

With recent advances in emerging Dynamic Spectrum Access (DSA) and Cognitive Radio technologies, modulation recognition (ModRec) has emerged as a critical problem with importance to spectrum-sharing applications. Existing approaches, target modulation recognition as if a packet will be decoded in full and thus, pose stringent requirements on spectrum sensing and transmitter behavior: (i) a transmitter's bandwidth should be scanned alone and in full, (ii) for MIMO ModRec, the sensor should have at least same as many antennas as the transmitter, (iii) modulation symbol representation should be uniform and (iv) prior knowledge of the transmitter's technology should be available. These stringent …


The Potential Impact Of Nuclear Conflict On Ocean Acidification, Nicole S. Lovenduski, Cheryl S. Harrison, Holly Olivarez, Charles G. Bardeen, Owen B. Toon, Joshua Coupe, Alan Robock, Tyler Rohr, Samantha Stevenson Jan 2020

The Potential Impact Of Nuclear Conflict On Ocean Acidification, Nicole S. Lovenduski, Cheryl S. Harrison, Holly Olivarez, Charles G. Bardeen, Owen B. Toon, Joshua Coupe, Alan Robock, Tyler Rohr, Samantha Stevenson

School of Earth, Environmental, and Marine Sciences Faculty Publications and Presentations

We demonstrate that the global cooling resulting from a range of nuclear conflict scenarios would temporarily increase the pH in the surface ocean by up to 0.06 units over a 5-year period, briefly alleviating the decline in pH associated with ocean acidification. Conversely, the global cooling dissolves atmospheric carbon into the upper ocean, driving a 0.1 to 0.3 unit decrease in the aragonite saturation state (Ωarag) that persists for ∼10 years. The peak anomaly in pH occurs 2 years post conflict, while the Ωarag anomaly peaks 4- to 5-years post conflict. The decrease in Ωarag would exacerbate a primary threat …


The Poisson Topp Leone Generator Of Distributions For Lifetime Data: Theory, Characterizations And Applications, Faton Merovci, Haitham M. Yousof, Gholamhossein Hamedani Jan 2020

The Poisson Topp Leone Generator Of Distributions For Lifetime Data: Theory, Characterizations And Applications, Faton Merovci, Haitham M. Yousof, Gholamhossein Hamedani

Mathematical and Statistical Science Faculty Research and Publications

We study a new family of distributions defined by the minimum of the Poisson random number of independent identically distributed random variables having a Topp Leone-G distribution (see Rezaei et al., (2016)). Some mathematical properties of the new family including ordinary and incomplete moments, quantile and generating functions, mean deviations, order statistics, reliability and entropies are derived. Maximum likelihood estimation of the model parameters is investigated. Some special models of the new family are discussed. An application is carried out on real data set applications sets to show the potentiality of the proposed family.


Global Research Productivity In Nuclear Waste Management: A Scientometric Analysis, Fayaz Ahmad Loan, Ufaira Yaseen Jan 2020

Global Research Productivity In Nuclear Waste Management: A Scientometric Analysis, Fayaz Ahmad Loan, Ufaira Yaseen

Library Philosophy and Practice (e-journal)

Scientometrics has emerged as one of the prominent and fast-growing fields in the Library and Information Sciences. The present study also deals with the scientometric aspect of one of the prominent fields of Nuclear Science and Technology i.e. Nuclear Waste Management. The data for the said study has been collected from the Web of Science database over the period 1989-2019. The results reveal that a total of 1824 publications have been published on Nuclear Waste Management and the highest number has been contributed by the USA (23.7%) of the total global output. Most of the Nuclear Waste Management literature …


Transformative Education In Agroecology: Student, Teacher, And Client Involvement In Co-Learning, Charles A. Francis, Anna Marie Nicolaysen, Geir Lieblein, Tor Arvid Breland Jan 2020

Transformative Education In Agroecology: Student, Teacher, And Client Involvement In Co-Learning, Charles A. Francis, Anna Marie Nicolaysen, Geir Lieblein, Tor Arvid Breland

Department of Agronomy and Horticulture: Faculty Publications

Educational methods have evolved rapidly in agroecology, which is a complex and holistic field without a long history or the formal tradition of any single academic discipline. Definitions of agroecology have evolved from its initial conception as a marriage of agriculture with ecology, to an aggregation of different paths including science, practices, and movements, and recently as a broad appreciation of the ecology of food systems. In contrast with traditional courses that begin with a history of the discipline and review the contributions of early leaders, we have embraced phenomenology to firmly establish roots in students’ learning through their experiences …


Bird And Native Bee Responses To Habitat Treatments, Emily Bea Oja Jan 2020

Bird And Native Bee Responses To Habitat Treatments, Emily Bea Oja

Graduate Student Theses, Dissertations, & Professional Papers

As forests across the United States have been altered due to fire suppression in the last century, their structure has been altered, resulting in increased fuel loads. Subsequently, managers have been increasingly implementing habitat treatments including prescribed burning, mechanical thinning, and a combination of both treatments to reduce fuel loads and enhance habitat for ungulates. The Rocky Mountain Elk Foundation has partnered with agencies to complete over 10,000 of these treatments across the United States to enhance elk habitat. As treatment impacts to other wildlife species are not well understood, we evaluated the effects of these treatments on the bird …


Tolle Lege Works Published In 2020, Mcquade Library Jan 2020

Tolle Lege Works Published In 2020, Mcquade Library

Bibliographies

Compiled Tolle Lege bibliography of works published by members of the Merrimack College Community in 2020. Works include journal articles, books, book chapters, conference presentations and posters, and more.


Nonlocal Means Estimation Of Intrinsic Mode Functions For Speech Enhancement, Sagar Reddy Vumanthala, Bikshalu K Jan 2020

Nonlocal Means Estimation Of Intrinsic Mode Functions For Speech Enhancement, Sagar Reddy Vumanthala, Bikshalu K

Turkish Journal of Electrical Engineering and Computer Sciences

The main aim of this paper is to introduce a new approach to enhance speech signals by exploring the advantages of nonlocal means (NLM) estimation and empirical mode decomposition. NLM, a patch-based denoising method, is extensively used for two-dimensional signals like images. However, its use for one-dimensional signals has been attracting more attention recently. The NLM-based approach is quite useful for removing low-frequency noises based on nonlocal similarities present among samples of the signal. However, there is an issue of under averaging in the high-frequency regions. The temporal and spectral characteristics of the speech signal are changing markedly over time. …


Multiplicative-Additive Despeckling In Sar Images, Gülay Aksoy, Fati̇h Nar Jan 2020

Multiplicative-Additive Despeckling In Sar Images, Gülay Aksoy, Fati̇h Nar

Turkish Journal of Electrical Engineering and Computer Sciences

Visual and automatic analyses using synthetic aperture radar (SAR) images are challenging because of inherently formed speckle noise. Thus, reducing speckle noise in SAR images is an important research area for SAR image analysis. During speckle noise reduction, homogeneous regions should be smoothed while details such as edges and point scatterers need to be preserved. General speckle noise model contains gamma distributed multiplicative part which is dominant and Gaussian distributed additive part which is in low amount and mostly neglected in literature. In this study, a novel sparsity-driven speckle reduction method is proposed that takes both multiplicative noise model and …


Detection Of Bga Solder Defects From X-Ray Images Using Deep Neural Network, Ceren Türer Akdeni̇z, Zümray Ölmez, Tamer Ölmez Jan 2020

Detection Of Bga Solder Defects From X-Ray Images Using Deep Neural Network, Ceren Türer Akdeni̇z, Zümray Ölmez, Tamer Ölmez

Turkish Journal of Electrical Engineering and Computer Sciences

In the literature it is observed that complex image processing operations are used in the classification of Ball Grid Array (BGA) X-ray images, however high classification results were not achieved. In recent years, it has been shown that deep learning methods are very successful especially in classification problems. In this study, a new deep neural network (DNN) model is proposed to classify the BGA X-ray images. The proposed DNN model contains feature extractor layers and a minimum distance classifier. Since the proposed network consists of less number of layers (4 convolution layers and 1 fully connected layer), determination of the …


Connectivity Considerations For Mission Planning Of A Search And Rescue Drone Team, Evşen Yanmaz Adam Jan 2020

Connectivity Considerations For Mission Planning Of A Search And Rescue Drone Team, Evşen Yanmaz Adam

Turkish Journal of Electrical Engineering and Computer Sciences

In this paper, we analyze the mission success performance and mission times of centralized, distributed, and hybrid path-planning methods for a drone team whose mission is to find a target and inform the ground control. We propose two methods that integrate connectivity into the search mission path decisions. We observe that even though the coverage path-planning leads to lower search times, when target connectivity is also required, schemes that incorporate end--end connectivity into path planning result in at least 50 % better mission times for small communication ranges and lower number of drones. Our results also indicate that methods to …


Fuzzy Genetic Based Dynamic Spectrum Allocation (Fgdsa) Approach For Cognitive Radio Sensor Networks, Ganesan Rajesh, Xavier Mercilin Raajini, Kulandairaj Martin Sagayam, Bharat Bhushan, Utku Kose Jan 2020

Fuzzy Genetic Based Dynamic Spectrum Allocation (Fgdsa) Approach For Cognitive Radio Sensor Networks, Ganesan Rajesh, Xavier Mercilin Raajini, Kulandairaj Martin Sagayam, Bharat Bhushan, Utku Kose

Turkish Journal of Electrical Engineering and Computer Sciences

Cognitive Radio Sensor Network (CRSN) is known as a distributed network of wireless cognitive radio sensor nodes. Such system senses an event signal and ensures collaborative dynamic communication processes over the spectrum bands. Here, the concept of Dynamic Spectrum Access (DSA) denes the method of reaching progressively to the unused range of spectrum band. As among the essential CRSN user types, the Primary User (PU) has the license to access the spectrum band. On the other hand, the Secondary User (SU) tries to access the unused spectrum eciently, by not disturbing the PU. Considering that issue, this study introduces a …


Wavelength Sensitivity Of Indium Tin Oxide On Surface Plasmon Resonance Angles, Antonio Ruiz, Carlos Villa Angulo, Ivan Olaf Hernandez-Fuentes Jan 2020

Wavelength Sensitivity Of Indium Tin Oxide On Surface Plasmon Resonance Angles, Antonio Ruiz, Carlos Villa Angulo, Ivan Olaf Hernandez-Fuentes

Turkish Journal of Electrical Engineering and Computer Sciences

Surface plasmon resonance (SPR) is a charge-density oscillation that occurs when a beam of p-polarized monochromatic light impinges with a greater angle than the critical angle in a dielectric-metal interface. Because of the high losses related to metals, the generated surface plasmon waves propagate with high attenuation in the visible and near-infrared spectral regions in most of the dielectric-metal interfaces. An alternative to reduce such losses is to use a transparent indium tin oxide (ITO) film. In this paper, we compared theoretical calculations and experimental measurements of the SPR angle $\theta_{SPR}$ on the interfaces of a borosilicate prism (Bp) and …


Mlcocoa: A Machine Learning-Based Congestion Control For Coap, Alper Kami̇l Demi̇r, Fati̇h Abut Jan 2020

Mlcocoa: A Machine Learning-Based Congestion Control For Coap, Alper Kami̇l Demi̇r, Fati̇h Abut

Turkish Journal of Electrical Engineering and Computer Sciences

Internet of Things (IoT) is a technological invention that has the potential to impact on how we live and how we work by connecting any device to the Internet. Consequently, a vast amount of novel applications will enhance our lives. Internet Engineering Task Force (IETF) standardized the Constrained Application Protocol (CoAP) to accommodate the application layer and network congestion needs of such IoT networks. CoAP is designed to be very simple where it employs a genuine congestion control (CC) mechanism, named as default CoAP CC leveraging basic binary exponential backoff. Yet efficient, default CoAP CC does not always utilize the …


Optimization Of Real-Time Wireless Sensor Based Big Data With Deep Autoencoder Network: A Tourism Sector Application With Distributed Computing, Beki̇r Aksoy, Utku Kose Jan 2020

Optimization Of Real-Time Wireless Sensor Based Big Data With Deep Autoencoder Network: A Tourism Sector Application With Distributed Computing, Beki̇r Aksoy, Utku Kose

Turkish Journal of Electrical Engineering and Computer Sciences

Internet usage has increased rapidly with the development of information communication technologies. The increase in internet usage led to the growth of data volumes on the internet and the emergence of the big data concept. Therefore, it has become even more important to analyze the data and make it meaningful. In this study, 690 million queries and approximately 5.9 quadrillion data collected daily from different servers were recorded on the Redis servers by using real-time big data analysis method and load balance structure for a company operating in the tourism sector. Here, wireless networks were used as a triggering factor …


Learning From Wilderness Fire: Restoring Landscape Scale Patterns And Processes, Julia Kittleson Berkey Jan 2020

Learning From Wilderness Fire: Restoring Landscape Scale Patterns And Processes, Julia Kittleson Berkey

Graduate Student Theses, Dissertations, & Professional Papers

Wilderness areas, because they are managed to be “untrammeled by man,” often offer the best approximation of intact, undisturbed ecological patterns and processes. In the case of wildland fire, this means that wilderness areas often provide the only landscapes where fire has been managed to play an active, ecosystem role. As a result, these wilderness areas offer unique lessons both in terms of wildland fire management as well as the ecological consequences that result from this management approach. For these reasons, an in-depth history of fire management in the wilderness areas of the Northern Rocky Mountains is provided to highlight …


Wind Power Forecasting Methods Based On Deep Learning: A Survey, Xing Deng, Haijian Shao, Chunlong Hu, Dengbiao Jiang, Yingtao Jiang Jan 2020

Wind Power Forecasting Methods Based On Deep Learning: A Survey, Xing Deng, Haijian Shao, Chunlong Hu, Dengbiao Jiang, Yingtao Jiang

Electrical & Computer Engineering Faculty Research

Accurate wind power forecasting in wind farm can effectively reduce the enormous impact on grid operation safety when high permeability intermittent power supply is connected to the power grid. Aiming to provide reference strategies for relevant researchers as well as practical applications, this paper attempts to provide the literature investigation and methods analysis of deep learning, enforcement learning and transfer learning in wind speed and wind power forecasting modeling. Usually, wind speed and wind power forecasting around a wind farm requires the calculation of the next moment of the definite state, which is usually achieved based on the state of …


Generating Peptide Mass Spectrometry Ground Truth Data, Jessica L. Henning, Rob Smith Jan 2020

Generating Peptide Mass Spectrometry Ground Truth Data, Jessica L. Henning, Rob Smith

Graduate Student Theses, Dissertations, & Professional Papers

Very few quantitative evaluations exist for precursor mass spectrometry data due to the lack of tools for enabling the manual feature finding necessary to generate this data. Other lacks the ability to capture, edit, save, and view precursor mass spectrometry data. We present JS-MS 2.0, a software suite that provides a dependency-free, browser-based, one click, cross-platform solution for creating precursor ground truth. The software retains the first version’s capacity for loading, viewing, and navigating MS1 data in 2- and 3-D, and adds tools for capturing, editing, saving and viewing isotopic envelope and extracted isotopic chromatogram features. The software can also …


Remote Sensing Approaches To Predict Forest Characteristics In Northwest Montana, Ryan P. Rock Jan 2020

Remote Sensing Approaches To Predict Forest Characteristics In Northwest Montana, Ryan P. Rock

Graduate Student Theses, Dissertations, & Professional Papers

Remote sensing can be utilized by land management organizations to save money and time. Mapping vegetation using either aerial photographs or satellite imagery and the applications for forest management are of particular interest to the Montana Department of Natural Resources. In 2018, the organization began a pilot program to test the incorporation of raster analysis of remotely sensed data into their inventory program and had limited success. This analysis identified two areas of improvement: the selection method of inventory plots and the imagery used for classification and metrics. This study found that selecting inventory plots using a generalized random tessellation …


Constructing Stable And Potentially High-Performance Hybrid Organic-Inorganic Perovskites With “Unstable” Cations, Qing Yang, Menghao Wu, Xiao Cheng Zeng Jan 2020

Constructing Stable And Potentially High-Performance Hybrid Organic-Inorganic Perovskites With “Unstable” Cations, Qing Yang, Menghao Wu, Xiao Cheng Zeng

Chemistry Department: Faculty Publications

A new family of functional hybrid organic-inorganic perovskites (HOIPs) is theoretically designed based on the following chemical+ insights: when a proton is adhered to molecules like water or ethanol, the newly formed larger-sized cations (e.g., H5O2 ,++ C2H5OH2 , and CH3SH ) entail low electron affinities mimicking superalkalis; they are conjugated acids of weak bases that cannot survive in solution, while their chemistry behavior in the HOIP frameworks, however, may be markedly different due to greatly enhanced cohesive energies of the proton, which facilitate the formation of new HOIPs. First-principles computations show that the putative formation reactions for these newly …


Domain Wall Conduction In Calcium-Modified Lead Titanate For Polarization Tunable Photovoltaic Devices, Chong-Xin Qian, Hong-Jian Hong-Jian, Qiang Zhang, Jiawei He, Zi-Xuan Chen, Ming-Zi Wang, Xiao Cheng Zeng Jan 2020

Domain Wall Conduction In Calcium-Modified Lead Titanate For Polarization Tunable Photovoltaic Devices, Chong-Xin Qian, Hong-Jian Hong-Jian, Qiang Zhang, Jiawei He, Zi-Xuan Chen, Ming-Zi Wang, Xiao Cheng Zeng

Chemistry Department: Faculty Publications

Ferroelectric domain wall (DW) conduction, confirmed in recent experiments, has attracted intense attention due to its promising applications in optoelec- tronic devices. Herein, we provide theoretical evidence of electric conduction in Pb0.8Ca0.2TiO3 (PCT) DWs. The separation of charge accumulation in DWs, corresponding to the electronic conduction-band minimum (CBM) and valence-band maximum (VBM), weakens the tendency for the electron-hole recombination, thereby providing more efficient channels for charge transfer. We fabricate PCT-based functional photovoltaic devices with polarization tunable charge transfer to exploit the combined conduction and ferroelectric properties of the DW. The photovoltaic performance of the devices can be regu- lated by …


Comparison Of Object Detection And Patch-Based Classification Deep Learning Models On Mid- To Late-Season Weed Detection In Uav Imagery, Arun Narenthiran Veeranampalayam Sivakumar, Jiating Li, Stephen Scott, Eric T. Psota, Amit J. Jhala, Joe D. Luck, Yeyin Shi Jan 2020

Comparison Of Object Detection And Patch-Based Classification Deep Learning Models On Mid- To Late-Season Weed Detection In Uav Imagery, Arun Narenthiran Veeranampalayam Sivakumar, Jiating Li, Stephen Scott, Eric T. Psota, Amit J. Jhala, Joe D. Luck, Yeyin Shi

Department of Biological Systems Engineering: Papers and Publications

Mid- to late-season weeds that escape from the routine early-season weed management threaten agricultural production by creating a large number of seeds for several future growing seasons. Rapid and accurate detection of weed patches in field is the first step of site-specific weed management. In this study, object detection-based convolutional neural network models were trained and evaluated over low-altitude unmanned aerial vehicle (UAV) imagery for mid- to late-season weed detection in soybean fields. The performance of two object detection models, Faster RCNN and the Single Shot Detector (SSD), were evaluated and compared in terms of weed detection performance using mean …


Self-Reported Data For Mental Workload Modelling In Human-Computer Interaction And Third-Level Education, Lucas Rizzo, Luca Longo Jan 2020

Self-Reported Data For Mental Workload Modelling In Human-Computer Interaction And Third-Level Education, Lucas Rizzo, Luca Longo

Articles

Mental workload (MWL) is an imprecise construct, with distinct definitions and no predominant measurement technique. It can be intuitively seen as the amount of mental activity devoted to a certain task over time. Several approaches have been proposed in the literature for the modelling and assessment of MWL. In this paper, data related to two sets of tasks performed by participants under different conditions is reported. This data was gathered from different sets of questionnaires answered by these participants. These questionnaires were aimed at assessing the features believed by domain experts to influence overall mental workload. In total, 872 records …


Road Network Simplification For Location-Based Services, Abdeltawab Hendawi, John A. Stankovic, Ayman Taha, Shaker El-Sappagh, Amr A. Ahmadain, Mohamed Ali Jan 2020

Road Network Simplification For Location-Based Services, Abdeltawab Hendawi, John A. Stankovic, Ayman Taha, Shaker El-Sappagh, Amr A. Ahmadain, Mohamed Ali

Articles

Road-network data compression or simplification reduces the size of the network to occupy less storage with the aim to fit small form-factor routing devices, mobile devices, or embedded systems. Simplification (a) reduces the storage cost of memory and disks, and (b) reduces the I/O and communication overhead. There are several road network compression techniques proposed in the literature. These techniques are evaluated by their compression ratios. However, none of these techniques takes into consideration the possibility that the generated compressed data can be used directly in Map-matching operation which is an essential component for all location-aware services. Map-matching matches a …


Are Electric Vehicles A Panacea For Reducing Ozone Precursor Emissions?, Gary A. Bishop Jan 2020

Are Electric Vehicles A Panacea For Reducing Ozone Precursor Emissions?, Gary A. Bishop

Fuel Efficiency Automobile Test Publications

No abstract provided.


A Molecular Dynamics Study Of Temperature Dependent Wetting In Alkane-Water Systems, Pauf Neupane Jan 2020

A Molecular Dynamics Study Of Temperature Dependent Wetting In Alkane-Water Systems, Pauf Neupane

Doctoral Dissertations

“The wetting behavior of aqueous organic systems is of great importance in several environmental and industrial processes such as the formation and growth of atmospheric aerosols, crude oil recovery from an oil field, onsite cleaning of natural gas, and clean-up of oil spills. In this work, we employed molecular dynamics (MD) simulations to explore the temperature dependent wetting behavior of octane and nonane on water in planar interfaces as well as in nanodroplets using PYS alkane and SPC/E and TIP4P/2005 water models.

For planar interfaces, we found unusual wetting behavior of octane and nonane on SPC/E water, but generally not …


Seismic Behavior Of Composite Bridge Columns, Mohanad M. Abdulazeez Jan 2020

Seismic Behavior Of Composite Bridge Columns, Mohanad M. Abdulazeez

Doctoral Dissertations

“This study investigates experimentally and numerically the seismic behavior of large-scale hollow-core fiber-reinforced polymer-concrete-steel (HC-FCS) innovative bridge columns as a sustainable approach to endure and rapidly recover from natural disasters such as earthquakes. The HC-FCS column consisted of a concrete shell sandwiched between an outer fiber-reinforced polymer (GFRP) tube and an inner steel tube to provided continuous confinement for the concrete shell along with the height of the column. The columns have a slender inner steel tube with diameter-to-thickness (Ds/ts) ratios ranged between 85 to 254. Each steel tube was embedded into the footing, while the …


Effect Of Subsurface Microseismicity On The Motion Of Surrounding Dispersed Droplets -- Data, Chao Zeng, Wen Deng Jan 2020

Effect Of Subsurface Microseismicity On The Motion Of Surrounding Dispersed Droplets -- Data, Chao Zeng, Wen Deng

Effect of Subsurface Microseismicity on the Motion of Surrounding Dispersed Droplets – Data

Spreadsheet - Data plotted in Figure 4 and Figure 5

Supporting information