Physical Sciences and Mathematics Commons^™

Electron Removal From Molecular Hydrogen By Fully Stripped Ions At Intermediate Energies, L. Meng, C. O. Reinhold, Ronald E. Olson

Physics Faculty Research & Creative Works

A classical phase-space model of the hydrogen molecule is presented and applied to the study of the electron-capture and -ionization processes in collisions of fully stripped ions with H2 at intermediate impact energies and charge states from 1 to 10. The model is based on the independent-electron and the impact-parameter approximations. The electron impinging-ion and electron target-nuclei interactions are exactly taken into account. The interaction between the electrons is approximated by model potentials. The calculated total cross sections for production of free electrons and capture of one electron are in good agreement with different experimental data. The ratio between the …

Mössbauer Effect Studies Of Nd₂Fe₁₄₋ₓsiₓb And Y₃Fe₁₄₋ₓsiₓb, Oran Allan Pringle, Gary J. Long, G. K. Marasinghe, William Joseph James, Antoni T. Pedziwiatr, W. E. Wallace, Fernande Grandjean

Physics Faculty Research & Creative Works

No abstract provided.

High-Temperature Defect Structure Of Nb-Doped Lacro3, Chikung J. Yu, Harlan U. Anderson, Don M. Sparlin

Materials Science and Engineering Faculty Research & Creative Works

Electrical conductivity and Seebeck measurements on LaCr_0.98Nb_0.02CrO₃ show that the defect structure of the material is mainly controlled by the extrinsic electrons formed by the Nb donors through the electronic compensation process. The experimental results also indicate that this material conducts electricity via a small polaron mechanism with an electron mobility around 0.004-0.01 cm2/V sec between 1100 and 1300°C. © 1989.

Oxidation-Reduction Behavior Of Undoped And Sr-Doped Lamno3 Nonstoichiometry And Defect Structure, J. H. Kuo, Harlan U. Anderson, Don M. Sparlin

Materials Science and Engineering Faculty Research & Creative Works

Undoped and Sr-doped LaMnO₃ showed reversible oxidation-reduction behavior. These perovskites can be excess, stoichiometric or deficient in oxygen content depending on the specific conditions. Under very reducing conditions decomposition into new phases occurs. Phase stabilities for these oxides were determined. The results showed that Sr doping caused the LaMnO₃ to dissociate at higher oxygen activities than those necessary for undoped LaMnO₃. Defect models are proposed to interpret the thermogravimetric results in which metal vacancies are assumed for the oxygen excess condition and oxygen vacancies are assumed for the oxygen deficient condition. Thermodynamic properties were calculated which …

Three-Body Interactions In Proton-Helium Angular Scattering, R. Dörner, J. Ullrich, H. Schmidt-Böcking, Ronald E. Olson

Physics Faculty Research & Creative Works

H⁺+He scattering at 0.5 MeV has been investigated using a coincidence technique that completely determines the three-body transverse momentum exchange in single ionization collisions. Three scattering regions could be distinctly recognized that are dominated by proton"helium-nucleus, proton-electron, or electron"helium-nucleus interactions. Calculations and the experimental data show that the coupling between the electronic and nuclear degrees of freedom is required to understand the dynamics for more than 97% of the ionizing collisions. © 1989 The American Physical Society.

Single- And Double-Ionization Cross Sections For Angular Scattering Of Fast Protons By Helium, R. (Ronald) E. Olson, J. Ullrich, R. Dörner, H. Schmidt-Böcking

Physics Faculty Research & Creative Works

The angular scattering of H⁺ by He has been investigated for single ionization at energies of 0.5, 1.0, and 3.0 MeV; and for double ionization at 1.0 MeV. The classical-trajectory Monte Carlo method has been used within one- and two-electron models to illustrate the collision dynamics. The angular differential single-ionization cross sections are in good agreement with experiment and display the combined effects of proton scattering from the He nucleus and its electrons. The relative fraction of double ionization, as a function of scattering angle, shows a maximum at 0.9 mrad that is in agreement with the experiments of …

Classical Two-Center Effects In Ejected-Electron Spectra From P+, P-, And He2++He Collisions At Intermediate Energies, C. O. Reinhold, Ronald E. Olson

Physics Faculty Research & Creative Works

Doubly and singly differential cross sections for electron emission have been calculated by means of the classical trajectory Monte Carlo method for the p⁺, p-, and He²⁺+He systems at impact energies of 50 and 100 keV/amu. The calculations for the p⁺ and He²⁺+He systems exhibit the capture to the continuum peak and agree in both shape and magnitude with experimental data. Analysis of the classical trajectories has helped to understand the dynamical formation of this peak. The dependence of the cross sections on the projectile charge (-1, +1, and +2) is analyzed and …

Theoretical Study Of Lattice Instabilities In Yba2Cu3O7, D. P. Billesbach, John R. Hardy, P. J. Edwardson

John R. Hardy Papers

We have performed a molecular dynamics simulation of the YBa₂Cu₃O₇ structure under the constraints of the rigid-ion model. These simulations used a variety of charge states for the Cu ions and the O ions, and except for one case, the interionic potentials were obtained in an ab initio fashion. The results of these simulations showed that a lattice instability involving the Cu-O chains existed. This instability was further investigated and it was shown that simple electronic screening is probably insufficient to stabilize the lattice. An instability of this nature provides a simple explanation of some …

Continuum Model Of Thin-Film Deposition And Growth, Andrew J. Bernoff, Seth Lichter

All HMC Faculty Publications and Research

A continuum theory for the deposition and growth of solid films is presented. The theory is developed in a coordinate-independent manner and so incorporates the fully nonlinear physics. The evolution of the film is modeled in three steps. First, the adsorption of atoms in the incident beam is modeled as a ballistic process. Second, the random motion of the adatoms is treated as a diffusive process. Finally, sticking of adatoms to the film occurs as a Poisson process. The resulting system of differential equations is examined in several parameter limits. The diffusively dominated limit appears similar to zone 1 of …

User-Friendly Model For The Energy Distribution Of Electrons From Proton Or Electron Collisions, M. Eugene Rudd

M. Eugene Rudd Publications

A model is presented which gives cross sections (differential in the ejected secondary electron energy) for the ionization of atoms and molecules in proton or electron collisions. The model is in the form of an analytical equation which holds for all primary and secondary energies and for any target gas for which certain parameters are known. The accuracy is estimated to be 15-20%. The model is based on the classical binary encounter model modified to agree with the Bethe theory at high energies and, for proton impact, with the molecular promotion model at low energies. For multi-shell targets, the partial …

Measured Spectra Of The Hygroscopic Fraction Of Atmospheric Aerosol Particles, Darryl J. Alofs, Donald E. Hagen, Max B. Trueblood

Mechanical and Aerospace Engineering Faculty Research & Creative Works

The Relation between Dry Diameter (Xo) and Critical Supersaturation (Sc) for Atmospheric Submicron Aerosol Particles is Investigated. the Particles Are Passed through an Electrostatic Aerosol Size Classifier, and Then through an Isothermal Haze Chamber. Results Are Reported in Terms of an Apparent Volume Fraction of Soluble Material, Εv, Defined Such that for Particles Composed Only of Ammonium Sulfate and Water Insoluble Compounds, Εv is the Actual Volume Fraction of Soluble Material. the Probability Distribution of Εv is Found to Be Approximately Gaussian in the Εv Range 0.2 to 1.3. the Mean Εv is 0.5, for Electrostatic Aerosol Classifier Settings of …

The Coupling Of Stimulated Raman And Brillouin Scattering In A Plasma, Donald P. Umstadter, W.B. Mori, C. Joshi

Donald Umstadter Publications

The observation of an anti-Stokes satellite in the spectrum of light backscattered from a CO₂ laser plasma is reported. Its origin is found to be Thomson scattering of the incident light from a counterpropagating mode-coupled plasma wave. The parent electron and ion waves in the mode-coupling process were driven by stimulated Raman and Brillouin backscattering. The parent and daughter plasma waves were detected by ruby laser Thomson scattering. A computer simulation modeling the experiment shows further cascading of the Stokes backscattered light to lower frequencies, apparently a result of its rescattering from another, higher phase velocity, counterpropagating coupled mode. …

Robert Katz: A Biographical Sketch, M. Eugene Rudd, John F. Fowler

Robert Katz Publications

Robert Katz was born in 1917 in New York City of Russian- Jewish immigrant parents. He grew up in the Bronx, attended Brooklyn College where he received his B.A. degree in 1937. A year later he was awarded the M.A. degree in physics at Columbia University. During World War II he worked for the Air Force at Wright Field in Ohio. After the war he returned to academia as a graduate student at the University of Illinois, where he earned the Ph.D. degree in physics in 1949. From that year he was a member of the Department of Physics at …

Analytically Reduced Form Of Multicenter Integrals From Gaussian Transforms, Jack C. Straton

Physics Faculty Publications and Presentations

In a previous paper the analytically reduced form was found for the general class of integrals containing multicenter products of ls hydrogenic orbitals, Coulomb or Yukawa potentials, and plane waves. The method consisted of combining all angular dependence within a single quadratic form by means of a three-dimensional Fourier transform and a one-dimensional Feynman transform for each term in the product and an additional integral transformation to move the resulting denominator into an exponential to be summed with the vector products in the plane waves. This quadratic form was then diagonalized with respect to the (introduced) momentum integrals and diagonalized …

Large-Angle Scattering In Positron-Helium And Positron-Krypton Collisions, D. R. Schultz, C. O. Reinhold, Ronald E. Olson

Physics Faculty Research & Creative Works

We have calculated differential cross sections as a function of the projectile scattering angle for positron-helium and positron-krypton collisions using the classical-trajectory Monte Carlo technique. These intermediate- velocity collisions have been simulated by various independent-electron and n-electron models, using both screened Coulomb and quantum model potentials to approximate the effects of electron-electron interactions. These several models all indicate that scattering of positrons to large angles in ionizing collisions persists to high impact velocities. In a previous work [Phys. Rev. A 38, 1866 (1988)] we proposed that the recent experiments that have measured the total cross section for positronium formation could …

Preliminary Results In Working With Molecular Modeling Software, Chris Hansen, Ray Hefferlin

Capstone Research Projects

In order to help facilitate the growing need for an understanding of periodic trends in molecules, an attempt was made to use a molecular modeling software package (ChemCad) to make a series of ab initio calculations of various properties of diaton1ic molecules. limitations of the package precluded calculations for strictly diatomic molecules, as well as precluding consecutive substitution of a large series of atoms into a larger molecule. This attempt does have significance in that it has allowed the physics department at Southern College to more effectively communicate with molecular modeling software developers and users.

A Study Of Oxygen Precipitation In Heavily Doped Silicon, Robert Kurt Graupner

Dissertations and Theses

Gettering of impurities with oxygen precipitates is widely used during the fabrication of semiconductors to improve the performance and yield of the devices. Since the effectiveness of the gettering process is largely dependent on the initial interstitial oxygen concentration, accurate measurements of this parameter are of considerable importance. Measurements of interstitial oxygen following thermal cycles are required for development of semiconductor fabrication processes and for research into the mechanisms of oxygen precipitate nucleation and growth. Efforts by industrial associations have led to the development of standard procedures for the measurement of interstitial oxygen in wafers. However practical oxygen measurements often …

Hamiltonian Formulation Of Induced Gravity In Two Dimensions, Charles G. Torre

All Physics Faculty Publications

A Hamiltonian formulation of the theory of induced gravity in two dimensions is constructed. This formulation differs from previous efforts in that the formalism is covariant under all relevant transformation groups. In particular, spatial diffeomorphism covariance and/or invariance is manifest throughout; the phase space carries a representation of the Lie algebra of the spacetime diffeomorphism group; the group of conformal isometries is projectively represented on the phase space as a symmetry group. The key ingredient that allows covariance with respect to the above groups is the enlargement of the gravitational phase space by the inclusion of the cotangent bundle over …

World Sheet Diffeomorphisms And The Canonical String, Charles G. Torre

All Physics Faculty Publications

The degree to which the phase space of a closed bosonic string carries a representation of the two‐dimensional diffeomorphism group Diff(M) is investigated. In particular, homomorphic mappings from the associated Lie algebra diff(M) into the Poisson algebra of functions on three natural phase spaces associated with the string are constructed. Two of these spaces are extended phase spaces based on the conformal and harmonic gauges, respectively. The third space is essentially the original phase space; the homomorphism in this case relies on the validity of the light‐cone gauge. Homomorphisms from diff(M) into the extended phase spaces of the Batalin–Fradkin–Vilkovisky formalism …

Ion Beam Mixing In Ag-Pd Alloys, J L. Klatt, R S. Averback, David Peak

All Physics Faculty Publications

Ion beam mixing during 750 keV Kr⁺ irradiation at 80 K was measured on a series of Ag‐Pd alloys using Au marker atoms. The mixing in pure Ag was the greatest and it decreased monotonically with increasing Pd content, being a factor of 10 higher in pure Ag than in pure Pd. This large difference in mixing cannot be explained by the difference in cohesion energy between Ag and Pd in the thermodynamic model of ion beam mixing proposed by Johnson et al. [W. L. Johnson, Y. T. Cheng, M. Van Rossum, and M‐A. Nicolet, Nucl. …

Theoretical Study Of The Seasonal Behavior Of The Global Ionosphere At Solar Maximum, Jan Josef Sojka, Robert W. Schunk

All Physics Faculty Publications

A time-dependent, three-dimensional, multi-ion numerical model of the global ionosphere was used to study the asymmetry in large-scale ionospheric features between the northern and southern hemispheres. The comparisons were done for June and December solstice conditions at solar maximum for quiet geomagnetic activity. Simple conditions and diurnally reproducible ionospheric features were established in order to elucidate the intrinsic hemispherical differences that are associated with the different displacements between the geomagnetic and geographic poles and the different atmospheric conditions. In comparing the ionospheric densities in the northern and southern hemispheres for a given season, we found the following: (1) The winter …

A Three-Dimensional Time-Dependent Model Of The Polar Wind, Robert W. Schunk, Jan Josef Sojka

All Physics Faculty Publications

A time-dependent global model of the polar wind was used to study transient polar wind perturbations during changing magnetospheric conditions. The model calculates three-dimensional distributions for the NO⁺, O₂⁺, N₂⁺, N⁺ and O⁺ densities and the ion and electron temperatures from diffusion and heat conduction equations at altitudes between 120 and 800 km. At altitudes above 500 km, the time-dependent nonlinear hydrodynamic equations for O⁺ and H⁺ are solved self-consistently with the ionospheric equations. The model takes account of supersonic ion outflow, shock formation, and ion energization during …

Modeled F Region Response To Auroral Dynamics Based Upon Dynamics Explorer Auroral Observations, Jan Josef Sojka, Robert W. Schunk, J. D. Cravens, L. A. Frank, J. Sharber, J. D. Winningham

All Physics Faculty Publications

Auroral images from the Dynamics Explorer 1 (DE 1) scanning auroral imager have been combined with in situ auroral precipitation data from the DE 2 low altitude plasma instrument to form a time-dependent global auroral energy flux model. This model has both good time (12 min) and spatial (100 km) resolution compared to that currently available for global scale ionospheric and thermospheric modeling. The development and comparison of this model with others are discussed. Data from an aurorally active period, November 25, 1981, are presented and used as a case study for this model. Using a global ionospheric model, the …

Thermospheric Dynamics During September 18-19, 1984, 2, Validation Of The Ncar Thermospheric General Circulation Model, G Crowley, B A. Emery, R G. Roble, H C. Carlson Jr., J E. Salah, Vincent B. Wickwar, K L. Miller, W L. Oliver, R G. Burnside, F A. Marcos

All Physics Faculty Publications

The validation of complex nonlinear numerical models such as the National Center for Atmospheric Research thermospheric general circulation model (NCAR TGCM) requires a detailed comparison of model predictions with data. The Equinox Transition Study (ETS) of September 17-24, 1984, provided a unique opportunity to address the verification of the NCAR TGCM, since unusually large quantities of high-quality thermospheric and ionospheric data were obtained during an intensive observation interval. In a companion paper (paper 1) by Crowley et al. (this issue) a simulation of the September 18-19 ETS interval was described. Using a novel approach to modeling, the TGCM inputs were …

Global Scale, Physical Models Of The F Region Ionosphere, Jan Josef Sojka

All Physics Faculty Publications

During the last decade, ionospheric F region modeling has reached an accurate climatological level. We now have global computer models of the F region which simulate the interactions between physical processes in the ionosphere. Because of their complexity, these climatological models are confined to modern day supercomputers. This review focuses on the development and verification of these physical ionospheric models. Such models are distinct from local models, steady state models, and empirical models of the ionosphere, which are, by their conception, unable to represent physically the range of F region variability or storm dynamics. This review examines the limitations of …

Mechanism Of Collisionally-Induced Transitions Among Fine-Structure Levels: Semiclassical Calculations Of Alignment Effects In The Na-He System, Laurie J. Kovalenko, Stephen R. Leone, John B. Delos

Arts & Sciences Articles

To gain insight into the mechanism of Na(3p)2P3/2→2P1/2 fine‐structure transitions induced by collision with He, we monitor the expectation values of the orbital‐ and spin‐angular momentum vectors, l and s, as a function of time along the trajectory, using a semiclassical formalism. In a typical collision, 〈s〉 remains nearly space‐fixed while 〈l〉 precesses about the rotating internuclear axis. Thus, in the interaction region, the projection of 〈l〉 onto the internuclear axis, 〈λ〉, remains nearly constant, and the molecular alignment of the orbital is preserved. We show how equations of motion for …

Calculations Of Scattered Light From Rigid Polymers By Shifrin And Rayleigh-Debye Approximations, M. F. Bishop

Physics Publications

ABSTRACT

We show that the commonly used Rayleigh-Debye method for calculating light scattering can lead to significant errors when used for describing scattering from dilute solutions of long rigid polymers, errors that can be overcome by use of the easily applied Shifrin approximation. In order to show the extent of the discrepancies between the two methods, we have performed calculations at normal incidence both for polarized and unpolarized incident light with the scattering intensity determined as a function of polarization angle and of scattering angle, assuming that the incident light is in a spectral region where the absorption of hemoglobin …

Optical And Electrochemical Studies Of Passive Film Formation In Amorphous Ni‐Cr‐P‐C Alloys, D. B. Hagan, B. W. Sloope, V. A. Niculescu

Physics Publications

The investigation of passivation of an amorphous Ni‐l4Cr‐17P‐0.5C alloy in lN H₂ SO₄ through anodic polarization and near‐normal optical reflectance is reported. It was found that the alloy passivates with a current density of 10^{− 1} A/m² extending to 1.0 V with current density dependent upon surface morphology. In the transpassive region under constant current density conditions the reflectance of the film exhibits strong interference phenomena and overall exponential decay in intensity. The behavior of the system in this region is described with a single thin‐film optical model consistent with the formation of a chromium …

Exciton Diffusion At Finite Frequency: Luminescence Observables For Anisotropic Percolating Solids, Paul Ernest Parris

Physics Faculty Research & Creative Works

A study is made of the luminescence intensities associated with exciton diffusion and trapping on a three-dimensional anisotropic percolating lattice. The calculation is based upon a relationship that exists between the frequency dependent diffusion tensor at frequencies comparable to the inverse excitation lifetime, and luminescence observables such as the host and trap luminescence intensities for conditions of constant illumination. The present approach allows the study of crossover behavior in percolative systems that are of intermediate transport dimensionality 2 < d_t < 3. Our results suggest that curvature seen in luminescence observables near the transition need not always be a direct reflection of the critical indices associated with classical isotropic percolation. We have identified three possible sources of deviation from the classical behavior: (1) the radiative time scale of the luminescence measurements, (2) the functional dependence of the luminescence yields on the diffusion tensor, and (3) the demands of dimensional crossover in the critical region arising from the anisotropy of the medium.

Strong Continuum-Continuum Couplings In The Direct Ionization Of Ar And He Atoms By 6-Mev/U U38+ And Th38+ Projectiles, D. Schneider, D. Dewitt, A. S. Schlachter, Ronald E. Olson, W. G. Graham, J. R. Mowat, R. (Robert) D. Dubois, D. H. Loyd, V. Montemayor, G. Schiwietz

Physics Faculty Research & Creative Works

Doubly differential cross sections have been measured as a function of the electron energy and observation angle for electron emission following collisions of 6-MeV/u U³⁸⁺ and Th³⁸⁺ on He and Ar. The electron-emission data show an enhancement at forward angles and a decrease at backward angles with respect to scaled-cross-section results based on the Born approximation. Comparison with classical-trajectory Monte Carlo calculations suggests that the deviation from the Born approximation can be explained by continuum-continuum couplings. By comparing with previously published data, we found that the forward enhancement as well as the backward decrease follow a q/vp (q,vp …